Department of Environmental Sciences and Engineering, University of North Carolina at Chapel Hill, Chapel Hill, North Carolina 27599, USA.
Covance CRS, LLC, Somerset, New Jersey 08873, USA.
Toxicol Sci. 2022 Jan 24;185(2):197-207. doi: 10.1093/toxsci/kfab140.
Vinyl acetate monomer (VAM) is heavily used to synthesize polymers. Previous studies have shown that inhaled VAM, being metabolized to acetaldehyde, may form DNA adducts including N2-ethylidene-deoxyguanosine (N2-EtD-dG), which may subsequently cause mutations and contribute to its carcinogenesis. Currently, there is little knowledge on the molecular dosimetry between VAM exposure and DNA adducts under dosages relevant to human exposure. In this study, 0.02, 0.1, 1, 10, 50, 200, and 600 ppm VAM were exposed to rats by inhalation for 14 days (6 h/day). The use of [13C2]-VAM allows unambiguous differentiation and quantification of the exogenous and endogenous N2-EtD-dG by highly sensitive LC-MS/MS. Our data indicate that VAM-induced exogenous DNA adducts were formed in a non-linear manner. Exogenous DNA adducts were only detected in the nasal epithelium of rats exposed to 10, 50, 200, and 600 ppm VAM, whereas endogenous adducts were found in all nasal and other tissues analyzed. In addition, ratios of exogenous/endogenous DNA adducts were less than 1 with the dose up to 50 ppm, indicating that endogenous DNA adducts are predominant at low VAM concentrations. Moreover, differential dose-response in terms of exogenous DNA adduct formation were observed between nasal respiratory and olfactory epithelium. Furthermore, the lack of exogenous DNA adducts in distant tissues, including peripheral blood mononuclear cells, liver, brain, and bone marrow, indicates that VAM and/or its metabolite do not distribute systemically to cause DNA damage in distant tissues. Together, these results provided new molecular dosimetry to improve science-based cancer risk assessments of VAM.
醋酸乙烯酯单体(VAM)被大量用于合成聚合物。先前的研究表明,吸入的 VAM 经代谢生成乙醛,可能会形成包括 N2-亚乙基-脱氧鸟苷(N2-EtD-dG)在内的 DNA 加合物,这些加合物可能随后导致突变,并促进其致癌作用。目前,对于与人类暴露相关剂量下 VAM 暴露与 DNA 加合物之间的分子剂量学知之甚少。在这项研究中,大鼠通过吸入暴露于 0.02、0.1、1、10、50、200 和 600 ppm 的 VAM 14 天(每天 6 小时)。使用 [13C2]-VAM 通过高灵敏度 LC-MS/MS 可以明确区分和定量外源性和内源性 N2-EtD-dG。我们的数据表明,VAM 诱导的外源性 DNA 加合物呈非线性形成。只有在暴露于 10、50、200 和 600 ppm VAM 的大鼠的鼻腔上皮中才检测到外源性 DNA 加合物,而在内源性 DNA 加合物在所有分析的鼻腔和其他组织中都有发现。此外,在外源/内源性 DNA 加合物的比值低于 1 时,直到 50 ppm 的剂量都小于 1,表明在低 VAM 浓度下内源性 DNA 加合物占主导地位。此外,在鼻腔呼吸和嗅觉上皮之间观察到外源性 DNA 加合物形成的差异剂量反应。此外,在外周血单核细胞、肝、脑和骨髓等远离组织中缺乏外源性 DNA 加合物表明 VAM 和/或其代谢物不会全身分布导致远离组织的 DNA 损伤。综上所述,这些结果为改进基于科学的 VAM 致癌风险评估提供了新的分子剂量学信息。