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单个量子点中的非线性下转换

Nonlinear down-conversion in a single quantum dot.

作者信息

Jonas B, Heinze D, Schöll E, Kallert P, Langer T, Krehs S, Widhalm A, Jöns K D, Reuter D, Schumacher S, Zrenner A

机构信息

Paderborn University, Physics Department, Warburger Straße 100, 33098, Paderborn, Germany.

Paderborn University, Center for Optoelectronics and Photonics Paderborn (CeOPP), Warburger Straße 100, 33098, Paderborn, Germany.

出版信息

Nat Commun. 2022 Mar 16;13(1):1387. doi: 10.1038/s41467-022-28993-3.

DOI:10.1038/s41467-022-28993-3
PMID:35297401
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC8927346/
Abstract

Tailored nanoscale quantum light sources, matching the specific needs of use cases, are crucial building blocks for photonic quantum technologies. Several different approaches to realize solid-state quantum emitters with high performance have been pursued and different concepts for energy tuning have been established. However, the properties of the emitted photons are always defined by the individual quantum emitter and can therefore not be controlled with full flexibility. Here we introduce an all-optical nonlinear method to tailor and control the single photon emission. We demonstrate a laser-controlled down-conversion process from an excited state of a semiconductor quantum three-level system. Based on this concept, we realize energy tuning and polarization control of the single photon emission with a control-laser field. Our results mark an important step towards tailored single photon emission from a photonic quantum system based on quantum optical principles.

摘要

量身定制的纳米级量子光源,能够满足特定用例的具体需求,是光子量子技术的关键组成部分。人们已经探索了几种不同的方法来实现高性能的固态量子发射器,并建立了不同的能量调谐概念。然而,发射光子的特性总是由单个量子发射器决定,因此无法完全灵活地控制。在此,我们介绍一种全光学非线性方法来定制和控制单光子发射。我们展示了一个由半导体量子三能级系统的激发态进行激光控制的下转换过程。基于这一概念,我们利用控制激光场实现了单光子发射的能量调谐和偏振控制。我们的结果标志着基于量子光学原理的光子量子系统实现量身定制单光子发射迈出了重要一步。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/d842ef9858fc/41467_2022_28993_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/be66dead4052/41467_2022_28993_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/aa2c4661ea28/41467_2022_28993_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/85b6c3fb7877/41467_2022_28993_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/00c8f22395a5/41467_2022_28993_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/bab92d4e9805/41467_2022_28993_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/d842ef9858fc/41467_2022_28993_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/be66dead4052/41467_2022_28993_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/aa2c4661ea28/41467_2022_28993_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/85b6c3fb7877/41467_2022_28993_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/00c8f22395a5/41467_2022_28993_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/bab92d4e9805/41467_2022_28993_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cf97/8927346/d842ef9858fc/41467_2022_28993_Fig6_HTML.jpg

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Nat Nanotechnol. 2021 Apr;16(4):399-403. doi: 10.1038/s41565-020-00831-x. Epub 2021 Jan 28.
2
Stimulated Raman Excited Fluorescence Spectroscopy and Imaging.受激拉曼激发荧光光谱学与成像
Nat Photonics. 2019 Jun;13(6):412-417. doi: 10.1038/s41566-019-0396-4. Epub 2019 Apr 1.
3
Scalable in operando strain tuning in nanophotonic waveguides enabling three-quantum-dot superradiance.可扩展的纳米光子波导内操作应变调谐实现三量子点超辐射
Nat Mater. 2019 Sep;18(9):963-969. doi: 10.1038/s41563-019-0418-0. Epub 2019 Jul 8.
4
High Purcell factor generation of indistinguishable on-chip single photons.高珀塞尔因子产生难以区分的片上单光子。
Nat Nanotechnol. 2018 Sep;13(9):835-840. doi: 10.1038/s41565-018-0188-x. Epub 2018 Jul 16.
5
Picosecond pulse shaping of single photons using quantum dots.利用量子点实现单光子的皮秒脉冲整形
Nat Commun. 2018 Jan 9;9(1):115. doi: 10.1038/s41467-017-02552-7.
6
High-performance semiconductor quantum-dot single-photon sources.高性能半导体量子点单光子源。
Nat Nanotechnol. 2017 Nov 7;12(11):1026-1039. doi: 10.1038/nnano.2017.218.
7
A quantum dot single-photon source with on-the-fly all-optical polarization control and timed emission.一种具有实时全光偏振控制和定时发射功能的量子点单光子源。
Nat Commun. 2015 Oct 5;6:8473. doi: 10.1038/ncomms9473.
8
Proposed robust and high-fidelity preparation of excitons and biexcitons in semiconductor quantum dots making active use of phonons.提出了一种利用声子在半导体量子点中制备稳健且高保真激子和双激子的方法。
Phys Rev Lett. 2013 Apr 5;110(14):147401. doi: 10.1103/PhysRevLett.110.147401. Epub 2013 Apr 2.
9
A dark-field microscope for background-free detection of resonance fluorescence from single semiconductor quantum dots operating in a set-and-forget mode.一种暗场显微镜,用于在“设定并遗忘”模式下对单个半导体量子点的共振荧光进行无背景检测。
Rev Sci Instrum. 2013 Jul;84(7):073905. doi: 10.1063/1.4813879.
10
On-demand semiconductor single-photon source with near-unity indistinguishability.按需半导体单光子源,具有近 100%的不可分辨性。
Nat Nanotechnol. 2013 Mar;8(3):213-7. doi: 10.1038/nnano.2012.262. Epub 2013 Feb 3.