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一种暗场显微镜,用于在“设定并遗忘”模式下对单个半导体量子点的共振荧光进行无背景检测。

A dark-field microscope for background-free detection of resonance fluorescence from single semiconductor quantum dots operating in a set-and-forget mode.

作者信息

Kuhlmann Andreas V, Houel Julien, Brunner Daniel, Ludwig Arne, Reuter Dirk, Wieck Andreas D, Warburton Richard J

机构信息

Department of Physics, University of Basel, Klingelbergstrasse 82, CH-4056 Basel, Switzerland.

出版信息

Rev Sci Instrum. 2013 Jul;84(7):073905. doi: 10.1063/1.4813879.

Abstract

Optically active quantum dots, for instance self-assembled InGaAs quantum dots, are potentially excellent single photon sources. The fidelity of the single photons is much improved using resonant rather than non-resonant excitation. With resonant excitation, the challenge is to distinguish between resonance fluorescence and scattered laser light. We have met this challenge by creating a polarization-based dark-field microscope to measure the resonance fluorescence from a single quantum dot at low temperature. We achieve a suppression of the scattered laser exceeding a factor of 10(7) and background-free detection of resonance fluorescence. The same optical setup operates over the entire quantum dot emission range (920-980 nm) and also in high magnetic fields. The major development is the outstanding long-term stability: once the dark-field point has been established, the microscope operates for days without alignment. The mechanical and optical designs of the microscope are presented, as well as exemplary resonance fluorescence spectroscopy results on individual quantum dots to underline the microscope's excellent performance.

摘要

例如自组装的铟镓砷量子点这类具有光学活性的量子点,有可能成为出色的单光子源。使用共振激发而非非共振激发时,单光子的保真度会有很大提高。在共振激发情况下,面临的挑战是区分共振荧光和散射激光。我们通过创建一台基于偏振的暗场显微镜来测量低温下单量子点的共振荧光,从而应对了这一挑战。我们实现了对散射激光的抑制超过10的7次方倍,并实现了共振荧光的无背景检测。同一光学装置可在整个量子点发射范围(920 - 980纳米)内运行,也能在强磁场中运行。主要进展在于出色的长期稳定性:一旦建立暗场点,显微镜无需校准即可运行数天。文中介绍了显微镜的机械和光学设计,以及单个量子点的典型共振荧光光谱结果,以突显显微镜的卓越性能。

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