Hashemi Mahdieh, Ansari Narges, Vazayefi Mahsa
Department of Physics, College of Science, Fasa University, Fasa, 74617-81189, Iran.
Department of Physics, Faculty of Physics and Chemistry, Alzahra University, Tehran, Iran.
Sci Rep. 2022 Apr 15;12(1):6313. doi: 10.1038/s41598-022-10280-2.
To design highly efficient and broadband nanometer-sized absorbers based on the atomically thin transition metal dichalcogenides (TMDCs), we propose utilizing inclined gold gratings on MoS monolayer. In the case of gold gratings with zero inclination, coverage of the absorption spectrum in the entire visible range occurs between the values of 42% to 73%. Considerable increase in the absorbed light occurs by introducing 13 nm inclination to the gold gratings with equal values of the grating's period and width as 60 nm. With the application of this grating, maximum absorption of 88% is reached and the absorption bandwidth covers the entire visible spectrum with only 12% variation of the absorption value relative to this maximum (88%). Footprints of resonant excitation of two different modes in the absorber structure are evident: the named "reflection" mode and localized surface plasmons (LSPs). Inclination of the gratings leads the LSP modes to slide toward the MoS and causes a remarkable increment in the absorption efficiency. An impressive absorption value of 56% in MoS monolayer is gained by the gold grating's inclination of 17 nm. The designed absorber paves a new way in designing TMDC-based absorbers with extended bandwidths and higher efficiencies.
为了基于原子级薄的过渡金属二硫化物(TMDCs)设计高效宽带纳米级吸收体,我们提出在单层MoS上利用倾斜的金光栅。对于倾斜度为零的金光栅,在整个可见光范围内吸收光谱的覆盖范围在42%至73%之间。通过对周期和宽度均为60nm的金光栅引入13nm的倾斜度,吸收的光量显著增加。应用这种光栅时,可实现88%的最大吸收率,且吸收带宽覆盖整个可见光谱,相对于该最大值(88%),吸收值的变化仅为12%。吸收体结构中两种不同模式的共振激发特征明显:即所谓的“反射”模式和局域表面等离子体(LSPs)。光栅的倾斜使LSP模式向MoS滑动,并导致吸收效率显著提高。通过17nm的金光栅倾斜度,单层MoS可获得56%的可观吸收率。所设计的吸收体为设计具有更宽带宽和更高效率的基于TMDC的吸收体开辟了一条新途径。