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多溴联苯醚 (PBDEs) 在海洋鱼类中的分布及纽芬兰的膳食暴露情况。

Polybrominated Diphenyl Ethers (PBDEs) in Marine Fish and Dietary Exposure in Newfoundland.

机构信息

Division of Community Health and Humanities, Faculty of Medicine, Memorial University, St. John's, NL, A1B 3V6, Canada.

Primary Healthcare Research Unit, Faculty of Medicine, Memorial University, St. John's, NL, A1B 3V6, Canada.

出版信息

Ecohealth. 2022 Mar;19(1):99-113. doi: 10.1007/s10393-022-01582-y. Epub 2022 Apr 26.

Abstract

Presence of PBDEs tested in 127 liver samples from Atlantic Cod (Gadus morhua) and Turbot (Scophthalmus Maximus) and 80 adult participants from two rural Newfoundland communities. Seafood consumption was measured through a validated seafood consumption questionnaire. PBDEs (-28, -47, -99, -156, and -209) were found in all fish liver samples, and PBB-153 and PBDEs-28, -47, -99, -100, -153 were identified as the most prominent congeners from the participants' serum samples. Cod was the most frequently consumed species in the seafood consumption survey. PBB-153 was higher amongst older (> 50 years age) participants (p < 0.0001), however, no PBDE congeners were significantly different by age. PBB-153 (p = 0.001), PBDE-153 (p = 0.006), and PBDE (p = 0.008) levels were significantly higher in males. The study shows that the marine ecosystem around Newfoundland has been contaminated by PBDEs, and that rural coastal residents are potentially exposed to these contaminants through local seafood consumption.

摘要

在来自纽芬兰两个农村社区的 80 名成年参与者和 127 个大西洋鳕鱼(Gadus morhua)和大菱鲆(Scophthalmus Maximus)肝脏样本中检测到 PBDEs。通过经过验证的海鲜消费问卷来衡量海鲜的消费情况。在所有的鱼肝样本中都发现了 PBDEs(-28、-47、-99、-156 和-209),并且从参与者的血清样本中确定了 PBB-153 和 PBDEs-28、-47、-99、-100、-153 为最主要的同系物。在海鲜消费调查中,鳕鱼是最常消费的物种。在年龄较大(>50 岁)的参与者中,PBB-153 含量更高(p<0.0001),但按年龄划分,没有 PBDE 同系物有显著差异。PBB-153(p=0.001)、PBDE-153(p=0.006)和 PBDE(p=0.008)水平在男性中明显更高。该研究表明,纽芬兰周围的海洋生态系统已受到 PBDEs 的污染,而当地的沿海居民可能通过当地的海鲜消费而接触到这些污染物。

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