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三维异质表面高光谱近场图像的快速模拟 - 第二部分

Rapid simulations of hyperspectral near-field images of three-dimensional heterogeneous surfaces - part II.

作者信息

Chen Xinzhong, Yao Ziheng, Sun Zhiyuan, Stanciu Stefan G, Basov D N, Hillenbrand Rainer, Liu Mengkun

出版信息

Opt Express. 2022 Mar 28;30(7):11228-11242. doi: 10.1364/OE.452949.

Abstract

The modeling of the near-field interaction in the scattering-type scanning near-field optical microscope (s-SNOM) is rapidly advancing, although an accurate yet versatile modeling framework that can be easily adapted to various complex situations is still lacking. In this work, we propose a time-efficient numerical scheme in the quasi-electrostatic limit to capture the tip-sample interaction in the near field. This method considers an extended tip geometry, which is a significant advantage compared to the previously reported method based on the point-dipole approximation. Using this formalism, we investigate, among others, nontrivial questions such as uniaxial and biaxial anisotropy in the near-field interaction, the relationship between various experimental parameters (e.g. tip radius, tapping amplitude, etc.), and the tip-dependent spatial resolution. The demonstrated method further sheds light on the understanding of the contrast mechanism in s-SNOM imaging and spectroscopy, while also representing a valuable platform for future quantitative analysis of the experimental observations.

摘要

散射型扫描近场光学显微镜(s-SNOM)中近场相互作用的建模正在迅速发展,尽管仍然缺乏一种准确且通用、能够轻松适应各种复杂情况的建模框架。在这项工作中,我们提出了一种在准静电极限下的高效数值方案,以捕捉近场中的针尖-样品相互作用。该方法考虑了扩展的针尖几何形状,与先前基于点偶极近似报道的方法相比,这是一个显著优势。使用这种形式体系,我们研究了诸多重要问题,如近场相互作用中的单轴和双轴各向异性、各种实验参数(如针尖半径、轻敲幅度等)之间的关系以及与针尖相关的空间分辨率。所展示的方法进一步有助于理解s-SNOM成像和光谱中的对比度机制,同时也为未来对实验观测进行定量分析提供了一个有价值的平台。

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