Huang Xiaohui, Li Riqiang, Duan Zhaozhao, Xu Fenfen, Li Hui
Jiangxi Provincial Key Laboratory of Functional Molecular Materials Chemistry, School of Chemistry and Chemical Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, P. R. China.
Soft Matter. 2022 May 25;18(20):3828-3844. doi: 10.1039/d2sm00352j.
Supramolecular polymer gels (SPGs) are precisely designed gels brought together by noncovalent interactions to form three-dimensional network structures of polymers. SPGs combine the merits of supramolecular polymers and gels, such as stimuli-responsiveness, self-healing, and self-adaptation, which endows SPGs with potential application value in the fields of biomaterials, Recently, much effort has been made to design new SPGs and related materials with high performance. Herein, we review the research endeavor and future directions of SPGs depending on the construction methods, topological structures, stimuli-responsiveness, and functionality. We hope that the review will provide reference values for the researchers working in supramolecular chemistry and gels.
超分子聚合物凝胶（SPGs）是通过非共价相互作用精确设计而成的凝胶，这些相互作用使聚合物形成三维网络结构。超分子聚合物凝胶结合了超分子聚合物和凝胶的优点，如刺激响应性、自愈性和自适应性，这赋予了超分子聚合物凝胶在生物材料领域潜在的应用价值。最近，人们在设计高性能的新型超分子聚合物凝胶及相关材料方面付出了很多努力。在此，我们根据构建方法、拓扑结构、刺激响应性和功能性对超分子聚合物凝胶的研究进展和未来方向进行综述。我们希望这篇综述能为从事超分子化学和凝胶研究的人员提供参考价值。
