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氧化石墨烯（GO）和还原氧化石墨烯（RGO）中间层在CZTSSe薄膜太阳能电池中的作用

The Role of the Graphene Oxide (GO) and Reduced Graphene Oxide (RGO) Intermediate Layer in CZTSSe Thin-Film Solar Cells.

作者信息

Jeong Woo-Lim, Park Sang-Hyuk, Jho Young-Dahl, Joo Soo-Kyung, Lee Dong-Seon

机构信息

School of Electrical Engineering and Computer Science, Gwangju Institute of Science and Technology, 123 Cheomdangwagi-ro, Gwangju 61005, Korea.

出版信息

Materials (Basel). 2022 May 10;15(10):3419. doi: 10.3390/ma15103419.

DOI:10.3390/ma15103419
PMID:35629447
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9144127/
Abstract

CuZnSn(S,Se) (CZTSSe) solar cells with low cost and eco-friendly characteristics are attractive as future sources of electricity generation, but low conversion efficiency remains an issue. To improve conversion efficiency, a method of inserting intermediate layers between the CZTSSe absorber film and the Mo back contact is used to suppress the formation of MoSe and decomposition of CZTSSe. Among the candidates for the intermediate layer, graphene oxide (GO) and reduced GO have excellent properties, including high-charge mobility and low processing cost. Depending on the type of GO, the solar cell parameters, such as fill factor (FF), were enhanced. Thus, the conversion efficiency of 6.3% was achieved using the chemically reduced GO intermediate layer with significantly improved FF.

摘要

具有低成本和环保特性的铜锌锡硫硒（CZTSSe）太阳能电池作为未来的发电来源很有吸引力，但转换效率低仍然是一个问题。为了提高转换效率，一种在CZTSSe吸收层薄膜和钼背接触之间插入中间层的方法被用来抑制MoSe的形成和CZTSSe的分解。在中间层的候选材料中，氧化石墨烯（GO）和还原氧化石墨烯具有优异的性能，包括高电荷迁移率和低加工成本。根据GO的类型，太阳能电池参数，如填充因子（FF）得到了提高。因此，使用化学还原的GO中间层实现了6.3%的转换效率，且FF有显著提高。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bc29/9144127/7e3d1729e5f7/materials-15-03419-g007.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bc29/9144127/4a5e9b08320a/materials-15-03419-g002.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/bc29/9144127/7e3d1729e5f7/materials-15-03419-g007.jpg

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