Wang Jing, Ma Jing, Huang Houbing, Ma Ji, Jafri Hasnain Mehdi, Fan Yuanyuan, Yang Huayu, Wang Yue, Chen Mingfeng, Liu Di, Zhang Jinxing, Lin Yuan-Hua, Chen Long-Qing, Yi Di, Nan Ce-Wen
Advanced Research Institute of Multidisciplinary Science, and School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, 100081, China.
State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084, China.
Nat Commun. 2022 Jun 6;13(1):3255. doi: 10.1038/s41467-022-30983-4.
The electronic conductivities of ferroelectric domain walls have been extensively explored over the past decade for potential nanoelectronic applications. However, the realization of logic devices based on ferroelectric domain walls requires reliable and flexible control of the domain-wall configuration and conduction path. Here, we demonstrate electric-field-controlled stable and repeatable on-and-off switching of conductive domain walls within topologically confined vertex domains naturally formed in self-assembled ferroelectric nano-islands. Using a combination of piezoresponse force microscopy, conductive atomic force microscopy, and phase-field simulations, we show that on-off switching is accomplished through reversible transformations between charged and neutral domain walls via electric-field-controlled domain-wall reconfiguration. By analogy to logic processing, we propose programmable logic gates (such as NOT, OR, AND and their derivatives) and logic circuits (such as fan-out) based on reconfigurable conductive domain walls. Our work might provide a potentially viable platform for programmable all-electric logic based on a ferroelectric domain-wall network with low energy consumption.
在过去十年中,人们对铁电畴壁的电导率进行了广泛研究,以探索其在潜在纳米电子应用中的可能性。然而,基于铁电畴壁的逻辑器件的实现需要对畴壁结构和传导路径进行可靠且灵活的控制。在此,我们展示了在自组装铁电纳米岛中自然形成的拓扑受限顶点域内,电场控制下导电畴壁的稳定且可重复的通断切换。通过结合压电力显微镜、导电原子力显微镜和相场模拟,我们表明通断切换是通过电场控制的畴壁重新配置,在带电畴壁和中性畴壁之间的可逆转变来实现的。类比逻辑处理,我们基于可重构导电畴壁提出了可编程逻辑门(如非门、或门、与门及其衍生物)和逻辑电路(如扇出电路)。我们的工作可能为基于低能耗铁电畴壁网络的可编程全电逻辑提供一个潜在可行的平台。