Department of Physics, Korea Advanced Institute of Science and Technology (KAIST), Yuseong-gu, Daejeon, 34141, Republic of Korea.
Department of Materials Modelling and Characterization, Korea Institute of Materials Science, Changwon, Gyeongnam, 51508, Republic of Korea.
Nat Commun. 2018 Jan 26;9(1):403. doi: 10.1038/s41467-017-02813-5.
Topological defects in matter behave collectively to form highly non-trivial structures called topological textures that are characterised by conserved quantities such as the winding number. Here we show that an epitaxial ferroelectric square nanoplate of bismuth ferrite subjected to a large strain gradient (as much as 10 m) associated with misfit strain relaxation enables five discrete levels for the ferroelectric topological invariant of the entire system because of its peculiar radial quadrant domain texture and its inherent domain wall chirality. The total winding number of the topological texture can be configured from - 1 to 3 by selective non-local electric switching of the quadrant domains. By using angle-resolved piezoresponse force microscopy in conjunction with local winding number analysis, we directly identify the existence of vortices and anti-vortices, observe pair creation and annihilation and manipulate the net number of vortices. Our findings offer a useful concept for multi-level topological defect memory.
物质中的拓扑缺陷集体表现为高度非平凡的结构,称为拓扑纹理,其特征是守恒量,如捻数。在这里,我们表明,由于其特殊的径向象限畴结构和固有畴壁手性,在与失配应变弛豫相关的大应变梯度(高达 10μm)下,铁电四方纳米板铋铁氧体可以实现整个系统的铁电拓扑不变量的五个离散能级。通过对角域的选择性非局域电开关,可以将拓扑纹理的总缠绕数配置为-1 到 3。通过结合角度分辨压电力显微镜和局部缠绕数分析,我们直接确定了涡旋和反涡旋的存在,观察到对的产生和湮灭,并操纵涡旋的净数量。我们的发现为多级拓扑缺陷存储器提供了一个有用的概念。