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棘轮胶体物质中的流体动力学同步与聚集

Hydrodynamic synchronization and clustering in ratcheting colloidal matter.

作者信息

Leyva Sergi G, Stoop Ralph L, Pagonabarraga Ignacio, Tierno Pietro

机构信息

Departament de Física de la Matèria Condensada, Universitat de Barcelona, Barcelona, Spain.

Universitat de Barcelona Institute of Complex Systems (UBICS), Universitat de Barcelona, Barcelona 08028, Spain.

出版信息

Sci Adv. 2022 Jun 10;8(23):eabo4546. doi: 10.1126/sciadv.abo4546. Epub 2022 Jun 8.

Abstract

Ratchet transport systems are widespread in physics and biology; however, the effect of the dispersing medium in the collective dynamics of these out-of-equilibrium systems has been often overlooked. We show that, in a traveling wave magnetic ratchet, long-range hydrodynamic interactions (HIs) produce a series of remarkable phenomena on the transport and assembly of interacting Brownian particles. We demonstrate that HIs induce the resynchronization with the traveling wave that emerges as a "speed-up" effect, characterized by a net raise of the translational speed, which doubles that of single particles. When competing with dipolar forces and the underlying substrate symmetry, HIs promote the formation of clusters that grow perpendicular to the driving direction. We support our findings both with Langevin dynamics and with a theoretical model that accounts for the fluid-mediated interactions. Our work illustrates the role of the dispersing medium on the dynamics of driven colloidal matter and unveils the growing process and cluster morphologies above a periodic substrate.

摘要

棘轮传输系统在物理学和生物学中广泛存在;然而,在这些非平衡系统的集体动力学中,分散介质的影响常常被忽视。我们表明,在行波磁性棘轮中,长程流体动力学相互作用(HIs)在相互作用的布朗粒子的传输和组装过程中产生了一系列显著现象。我们证明,HIs 会导致与行波重新同步,这表现为一种“加速”效应,其特征是平移速度的净提高,这是单个粒子速度的两倍。当与偶极力和底层衬底对称性竞争时,HIs 促进了垂直于驱动方向生长的团簇的形成。我们通过朗之万动力学和一个考虑流体介导相互作用的理论模型来支持我们的发现。我们的工作阐明了分散介质在驱动胶体物质动力学中的作用,并揭示了周期性衬底上方的生长过程和团簇形态。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/56ef/9177066/f67a13463803/sciadv.abo4546-f1.jpg

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