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钙钛矿金属包覆层中电注入激子极化激元的定向发射。

Directional Emission from Electrically Injected Exciton-Polaritons in Perovskite Metasurfaces.

机构信息

Centre for Disruptive Photonic Technologies, TPI, Nanyang Technological University, 21 Nanyang Link, Singapore 637371.

Interdisciplinary Graduate School, Energy Research Institute @NTU (ERI@N), Nanyang Technological University, 50 Nanyang Drive, Singapore 637553.

出版信息

Nano Lett. 2023 May 24;23(10):4431-4438. doi: 10.1021/acs.nanolett.3c00727. Epub 2023 May 2.

Abstract

We present a new approach to achieving strong coupling between electrically injected excitons and photonic bound states in the continuum of a dielectric metasurface. Here a high-finesse metasurface cavity is monolithically patterned in the channel of a perovskite light-emitting transistor to induce a large Rabi splitting of ∼200 meV and more than 50-fold enhancement of the polaritonic emission compared to the intrinsic excitonic emission of the perovskite film. Moreover, the directionality of polaritonic electroluminescence can be dynamically tuned by varying the source-drain bias, which induces an asymmetric distribution of exciton population within the transistor channel. We argue that this approach provides a new platform to study strong light-matter interactions in dispersion engineered photonic cavities under electrical injection and paves the way to solution-processed electrically pumped polariton lasers.

摘要

我们提出了一种新方法,可在介电超表面的连续体中实现电注入激子与光子束缚态之间的强耦合。在这里,通过在钙钛矿发光晶体管的沟道中整体图案化高精细度超表面腔,可诱导出约 200 meV 的大拉比分裂,并且与钙钛矿薄膜的本征激子发射相比,可增强超过 50 倍的极化激元发射。此外,通过改变源漏偏压可以动态调节极化激子电致发光的方向性,这会导致晶体管沟道内激子分布的不对称。我们认为,这种方法为在电注入下研究经色散工程处理的光子腔中的强光物质相互作用提供了一个新平台,并为溶液处理的电泵浦极化激子激光器铺平了道路。

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