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有机-无机卤化物钙钛矿中的室温极化子软自旋XY哈密顿量

Room temperature polaritonic soft-spin XY Hamiltonian in organic-inorganic halide perovskites.

作者信息

Peng Kai, Li Wei, Berloff Natalia G, Zhang Xiang, Bao Wei

机构信息

Department of Materials Science and Engineering, Rensselaer Polytechnic Institute, Troy, NY, USA.

Nanoscale Science and Engineering Center, University of California, Berkeley, CA, USA.

出版信息

Nanophotonics. 2024 Feb 15;13(14):2651-2658. doi: 10.1515/nanoph-2023-0818. eCollection 2024 Jun.

Abstract

Exciton-polariton condensates, due to their nonlinear and coherent characteristics, have been employed to construct spin Hamiltonian lattices for potentially studying spin glass, critical dephasing, and even solving optimization problems. Here, we report the room-temperature polariton condensation and polaritonic soft-spin XY Hamiltonian lattices in an organic-inorganic halide perovskite microcavity. This is achieved through the direct integration of high-quality single-crystal samples within the cavity. The ferromagnetic and antiferromagnetic couplings in both one- and two-dimensional condensate lattices have been observed clearly. Our work shows a nonlinear organic-inorganic hybrid perovskite platform for future investigations as polariton simulators.

摘要

由于激子极化激元具有非线性和相干特性,它们已被用于构建自旋哈密顿晶格,以潜在地研究自旋玻璃、临界退相,甚至解决优化问题。在此,我们报告了在有机-无机卤化物钙钛矿微腔中实现的室温极化激元凝聚和极化激元软自旋XY哈密顿晶格。这是通过将高质量的单晶样品直接集成到微腔内实现的。在一维和二维凝聚晶格中都清晰地观察到了铁磁和反铁磁耦合。我们的工作展示了一个用于未来作为极化激元模拟器进行研究的非线性有机-无机混合钙钛矿平台。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/340e/11636516/0a0109c2736f/j_nanoph-2023-0818_fig_001.jpg

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