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使用生物复合吸附剂从水溶液中去除纺织染料

The Removal of a Textile Dye from an Aqueous Solution Using a Biocomposite Adsorbent.

作者信息

Ferkous Hana, Rouibah Karima, Hammoudi Nour-El-Houda, Alam Manawwer, Djilani Chahrazed, Delimi Amel, Laraba Omar, Yadav Krishna Kumar, Ahn Hyun-Jo, Jeon Byong-Hun, Benguerba Yacine

机构信息

Laboratoire de Génie Mécanique et Matériaux, Faculté de Technologie, Université de 20 Août 1955, Skikda 21000, Algeria.

Département de Technologie, Université de 20 Août 1955 de Skikda, Skikda 21000, Algeria.

出版信息

Polymers (Basel). 2022 Jun 13;14(12):2396. doi: 10.3390/polym14122396.

DOI:10.3390/polym14122396
PMID:35745972
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9227792/
Abstract

The adsorption mechanisms of methylene blue (MB) onto olive waste (residue) treated with KOH (OR-KOH) and onto an OR-KOH and PEG-silica gel composite (OR-KOH/PEG-SG) at various temperatures were investigated using a combination of experimental analysis and Monte Carlo ab-initio simulations. The effects of adsorption process variables such as pH, temperature, and starting adsorbate concentration were investigated. The experimental data were fitted to Langmuir and Freundlich models. The maximum adsorption capacities of MB onto OR-KOH and OR-KOH/PEG-SG adsorbents reached values of 504.9 mg/g and 161.44 mg/g, respectively. The experimental FT-IR spectra indicated that electrostatic attraction and hydrogen bond formation were critical for MB adsorption onto the adsorbents generated from olive waste. The energetic analyses performed using Monte Carlo atomistic simulations explained the experimental results of a differential affinity for the investigated adsorbents and confirmed the nature of the interactions between methylene blue and the adsorbents to be van der Waals electrostatic forces.

摘要

采用实验分析和蒙特卡罗从头算模拟相结合的方法，研究了亚甲基蓝（MB）在不同温度下在经KOH处理的橄榄渣（残渣）（OR-KOH）以及OR-KOH与聚乙二醇-硅胶复合材料（OR-KOH/PEG-SG）上的吸附机制。研究了吸附过程变量如pH值、温度和起始吸附质浓度的影响。将实验数据拟合到朗缪尔和弗伦德利希模型。MB在OR-KOH和OR-KOH/PEG-SG吸附剂上的最大吸附容量分别达到504.9 mg/g和161.44 mg/g。实验傅里叶变换红外光谱表明，静电吸引和氢键形成对于MB在橄榄渣产生的吸附剂上的吸附至关重要。使用蒙特卡罗原子模拟进行的能量分析解释了所研究吸附剂具有不同亲和力的实验结果，并证实亚甲基蓝与吸附剂之间的相互作用性质为范德华静电力。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/25e85265b60d/polymers-14-02396-g007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/f5ff4a6bd2d6/polymers-14-02396-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/b06c14dd99ad/polymers-14-02396-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/3a818b601fc9/polymers-14-02396-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/bca9525d473b/polymers-14-02396-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/97284e4706aa/polymers-14-02396-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/5cd125a624a9/polymers-14-02396-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/25e85265b60d/polymers-14-02396-g007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/f5ff4a6bd2d6/polymers-14-02396-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/b06c14dd99ad/polymers-14-02396-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/3a818b601fc9/polymers-14-02396-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/bca9525d473b/polymers-14-02396-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/97284e4706aa/polymers-14-02396-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/5cd125a624a9/polymers-14-02396-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3e63/9227792/25e85265b60d/polymers-14-02396-g007.jpg

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