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通过塞曼分裂测量揭示的WS₂单层中的应变诱导激子杂化

Strain-Induced Exciton Hybridization in WS_{2} Monolayers Unveiled by Zeeman-Splitting Measurements.

作者信息

Blundo Elena, Junior Paulo E Faria, Surrente Alessandro, Pettinari Giorgio, Prosnikov Mikhail A, Olkowska-Pucko Katarzyna, Zollner Klaus, Woźniak Tomasz, Chaves Andrey, Kazimierczuk Tomasz, Felici Marco, Babiński Adam, Molas Maciej R, Christianen Peter C M, Fabian Jaroslav, Polimeni Antonio

机构信息

Physics Department, Sapienza University of Rome, 00185 Rome, Italy.

Institute for Theoretical Physics, University of Regensburg, 93040 Regensburg, Germany.

出版信息

Phys Rev Lett. 2022 Aug 5;129(6):067402. doi: 10.1103/PhysRevLett.129.067402.

Abstract

Mechanical deformations and ensuing strain are routinely exploited to tune the band gap energy and to enhance the functionalities of two-dimensional crystals. In this Letter, we show that strain leads also to a strong modification of the exciton magnetic moment in WS_{2} monolayers. Zeeman-splitting measurements under magnetic fields up to 28.5 T were performed on single, one-layer-thick WS_{2} microbubbles. The strain of the bubbles causes a hybridization of k-space direct and indirect excitons resulting in a sizable decrease in the modulus of the g factor of the ground-state exciton. These findings indicate that strain may have major effects on the way the valley number of excitons can be used to process binary information in two-dimensional crystals.

摘要

机械变形及随之产生的应变常被用于调节带隙能量并增强二维晶体的功能。在本信函中,我们表明应变还会导致二硫化钨(WS₂)单层中激子磁矩的强烈改变。我们对单层厚的WS₂单个微泡施加高达28.5特斯拉的磁场进行塞曼分裂测量。微泡的应变导致k空间直接和间接激子发生杂化,致使基态激子的g因子模量大幅降低。这些发现表明,应变可能对利用激子谷数在二维晶体中处理二进制信息的方式产生重大影响。

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