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用于药物修复和病原体灭活的Z型光催化剂的调控:设计贡献、概念检验及进展

Modulation of Z-scheme photocatalysts for pharmaceuticals remediation and pathogen inactivation: Design devotion, concept examination, and developments.

作者信息

Edwin Malefane Mope, John Mafa Potlako, Thokozani Innocent Nkambule Thabo, Elizabeth Managa Muthumuni, Tawanda Kuvarega Alex

机构信息

Institute for Nanotechnology and Water Sustainability, College of Science, Engineering and Technology, University of South Africa, Florida 1709, Johannesburg, South Africa.

出版信息

Chem Eng J. 2023 Jan 15;452:138894. doi: 10.1016/j.cej.2022.138894. Epub 2022 Aug 29.

Abstract

The recent outbreak of Covid-19 guarantees overconsumption of different drugs as a necessity to reduce the symptoms caused by this pandemic. This triggers the proliferation of pharmaceuticals into drinking water systems. Is there any hope for access to safe drinking water? Photocatalytic degradation using artificial Z-scheme photocatalysts that has been employed for over a decade conveys a prospect for sustainable clean water supply. It is compelling to comprehensively summarise the state-of-the-art effects of Z-scheme photocatalytic systems towards the removal of pharmaceuticals in water. The principle of Z-scheme and the techniques used to validate the Z-scheme interfacial charge transfer are explored in detail. The application of the Z-scheme photocatalysts towards the degradation of antibiotics, NSAIDs, and bacterial/viral inactivation is deliberated. Conclusions and stimulating standpoints on the challenges of this emergent research direction are presented. The insights and up-to-date information will prompt the up-scaling of Z- scheme photocatalytic systems for commercialization.

摘要

近期新冠疫情的爆发使得人们为减轻这一流行病引发的症状而过度使用各类药物成为必要。这引发了药品向饮用水系统的扩散。获取安全饮用水还有希望吗?使用人工Z型光催化剂进行光催化降解已应用了十多年,为可持续的清洁水供应带来了前景。全面总结Z型光催化系统在去除水中药物方面的最新效果很有必要。详细探讨了Z型原理以及用于验证Z型界面电荷转移的技术。审议了Z型光催化剂在抗生素降解、非甾体抗炎药降解以及细菌/病毒灭活方面的应用。针对这一新兴研究方向的挑战给出了结论和具有启发性的观点。这些见解和最新信息将促使Z型光催化系统扩大规模以实现商业化。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c88/9422400/ad6f34494800/ga1_lrg.jpg

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