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可持续生物炭活化过硫酸盐去除抗生素的综述

A Mini Review on Persulfate Activation by Sustainable Biochar for the Removal of Antibiotics.

作者信息

Li Mengxue, Li Peng, Zhou Qi, Lee Stephanie Ling Jie

机构信息

College of Environmental Science and Engineering, Tongji University, Shanghai 200092, China.

Australian Institute for Bioengineering and Nanotechnology, The University of Queensland, Brisbane, QLD 4072, Australia.

出版信息

Materials (Basel). 2022 Aug 24;15(17):5832. doi: 10.3390/ma15175832.

Abstract

Antibiotic contamination in water bodies poses ecological risks to aquatic organisms and humans and is a global environmental issue. Persulfate-based advanced oxidation processes (PS-AOPs) are efficient for the removal of antibiotics. Sustainable biochar materials have emerged as potential candidates as persulfates (Peroxymonosulfate (PMS) and Peroxydisulfate (PDS)) activation catalysts to degrade antibiotics. In this review, the feasibility of pristine biochar and modified biochar (non-metal heteroatom-doped biochar and metal-loaded biochar) for the removal of antibiotics in PS-AOPs is evaluated through a critical analysis of recent research. The removal performances of biochar materials, the underlying mechanisms, and active sites involved in the reactions are studied. Lastly, sustainability considerations for future biochar research, including Sustainable Development Goals, technical feasibility, toxicity assessment, economic and life cycle assessment, are discussed to promote the large-scale application of biochar/PS technology. This is in line with the global trends in ensuring sustainable production.

摘要

水体中的抗生素污染对水生生物和人类构成生态风险,是一个全球性环境问题。基于过硫酸盐的高级氧化工艺(PS-AOPs)对去除抗生素很有效。可持续生物炭材料已成为潜在的过硫酸盐(过一硫酸盐(PMS)和过二硫酸盐(PDS))活化催化剂以降解抗生素的候选材料。在本综述中,通过对近期研究的批判性分析,评估了原始生物炭和改性生物炭(非金属杂原子掺杂生物炭和负载金属生物炭)在PS-AOPs中去除抗生素的可行性。研究了生物炭材料的去除性能、潜在机制以及反应中涉及的活性位点。最后,讨论了未来生物炭研究的可持续性考量,包括可持续发展目标、技术可行性、毒性评估、经济和生命周期评估,以促进生物炭/PS技术的大规模应用。这符合确保可持续生产的全球趋势。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9dd2/9456675/ee95b5f81396/materials-15-05832-g001.jpg

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