Department of Chemistry, Institute for Chemical Epigenetics, Ludwig-Maximilians-Universität München, Würmtalstr. 201, 81375, Munich, Germany.
Faculty of Chemistry, Technical University of Munich, Lichtenbergstr. 4, 85748, Garching, Germany.
Clin Epigenetics. 2022 Sep 11;14(1):113. doi: 10.1186/s13148-022-01329-0.
Azacytidine (AzaC) and decitabine (AzadC) are cytosine analogs that covalently trap DNA methyltransferases, which place the important epigenetic mark 5-methyl-2'-deoxycytidine by methylating 2'-deoxycytidine (dC) at the C5 position. AzaC and AzadC are used in the clinic as antimetabolites to treat myelodysplastic syndrome and acute myeloid leukemia and are explored against other types of cancer. Although their principal mechanism of action is known, the downstream effects of AzaC and AzadC treatment are not well understood and the cellular prerequisites that determine sensitivity toward AzaC and AzadC remain elusive. Here, we investigated the effects and phenotype of AzaC and AzadC exposure on the acute myeloid leukemia cell line MOLM-13. We found that while AzaC and AzadC share many effects on the cellular level, including decreased global DNA methylation, increased formation of DNA double-strand breaks, transcriptional downregulation of important oncogenes and similar changes on the proteome level, AzaC failed in contrast to AzadC to induce apoptosis efficiently in MOLM-13. The only cellular marker that correlated with this clear phenotypical outcome was the level of hydroxy-methyl-dC, an additional epigenetic mark that is placed by TET enzymes and repressed in cancer cells. Whereas AzadC increased hmdC substantially in MOLM-13, AzaC treatment did not result in any increase at all. This suggests that hmdC levels in cancer cells should be monitored as a response toward AzaC and AzadC and considered as a biomarker to judge whether AzaC or AzadC treatment leads to cell death in leukemic cells.
阿扎胞苷(AzaC)和地西他滨(AzadC)是胞嘧啶类似物,可通过将 2'-脱氧胞苷(dC)的 C5 位甲基化来共价捕获 DNA 甲基转移酶,从而产生重要的表观遗传标记 5-甲基-2'-脱氧胞苷。AzaC 和 AzadC 临床上用作抗代谢物治疗骨髓增生异常综合征和急性髓细胞白血病,并针对其他类型的癌症进行探索。尽管它们的主要作用机制已经明确,但 AzaC 和 AzadC 治疗的下游效应尚未得到很好的理解,决定对 AzaC 和 AzadC 敏感性的细胞前提条件仍难以捉摸。在这里,我们研究了 AzaC 和 AzadC 暴露对急性髓细胞白血病细胞系 MOLM-13 的影响和表型。我们发现,虽然 AzaC 和 AzadC 在细胞水平上有许多共同的作用,包括降低全基因组 DNA 甲基化、增加 DNA 双链断裂的形成、重要癌基因的转录下调以及蛋白质组水平的类似变化,但与 AzadC 相反,AzaC 不能有效地诱导 MOLM-13 细胞凋亡。与这一明显表型结果相关的唯一细胞标记是羟甲基-dC 的水平,羟甲基-dC 是一种额外的表观遗传标记,由 TET 酶放置并在癌细胞中受到抑制。虽然 AzadC 使 MOLM-13 中的 hmdC 显著增加,但 AzaC 处理根本没有导致任何增加。这表明应将癌细胞中的 hmdC 水平作为对 AzaC 和 AzadC 的反应进行监测,并将其视为判断 AzaC 或 AzadC 治疗是否导致白血病细胞死亡的生物标志物。