Brown Timothy D, Bohaichuk Stephanie M, Islam Mahnaz, Kumar Suhas, Pop Eric, Williams R Stanley
Department of Electrical and Computer Engineering, Texas A&M University, College Station, TX, 77843, USA.
Sandia National Laboratories, Livermore, CA, 94550, USA.
Adv Mater. 2023 Sep;35(37):e2205451. doi: 10.1002/adma.202205451. Epub 2022 Nov 3.
Translating the surging interest in neuromorphic electronic components, such as those based on nonlinearities near Mott transitions, into large-scale commercial deployment faces steep challenges in the current lack of means to identify and design key material parameters. These issues are exemplified by the difficulties in connecting measurable material properties to device behavior via circuit element models. Here, the principle of local activity is used to build a model of VO /SiN Mott threshold switches by sequentially accounting for constraints from a minimal set of quasistatic and dynamic electrical and high-spatial-resolution thermal data obtained via in situ thermoreflectance mapping. By combining independent data sets for devices with varying dimensions, the model is distilled to measurable material properties, and device scaling laws are established. The model can accurately predict electrical and thermal conductivities and capacitances and locally active dynamics (especially persistent spiking self-oscillations). The systematic procedure by which this model is developed has been a missing link in predictively connecting neuromorphic device behavior with their underlying material properties, and should enable rapid screening of material candidates before employing expensive manufacturing processes and testing procedures.
将对神经形态电子元件(如基于莫特转变附近非线性特性的元件)的激增兴趣转化为大规模商业应用,在当前缺乏识别和设计关键材料参数的手段的情况下面临严峻挑战。这些问题体现在通过电路元件模型将可测量的材料特性与器件行为联系起来存在困难。在此,利用局部活性原理,通过依次考虑从通过原位热反射映射获得的一组最小的准静态和动态电学及高空间分辨率热数据的约束条件,构建了VO /SiN莫特阈值开关模型。通过结合不同尺寸器件的独立数据集,将模型提炼为可测量的材料特性,并建立了器件缩放定律。该模型能够准确预测电导率、热导率和电容以及局部活性动力学(特别是持续的尖峰自振荡)。开发此模型的系统程序一直是将神经形态器件行为与其基础材料特性进行预测性联系中缺失的环节,并且应该能够在采用昂贵的制造工艺和测试程序之前快速筛选候选材料。