Putman Annie L, Jones Daniel K, Blakowski Molly A, DiViesti Destry, Hynek Scott A, Fernandez Diego P, Mendoza Daniel
Utah Water Science Center U.S. Geological Survey West Valley City UT USA.
Department of Watershed Sciences Utah State University Logan UT USA.
Geohealth. 2022 Nov 1;6(11):e2022GH000671. doi: 10.1029/2022GH000671. eCollection 2022 Nov.
The Salt Lake Valley, UT, USA, is proximal to the desiccating Great Salt Lake (GSL). Prior work has found that this lakebed/playa contributes metals-laden dust to snow in the Wasatch and Uinta Mountains. Dust and industrial particulate pollution are also delivered to communities along the Wasatch Front, but their sources, compositions, and fluxes are poorly characterized. In this study, we analyzed the dust deposited in 18 passive samplers positioned near the GSL, in cities in and near the Salt Lake Valley for total dust flux, the <63 µm dust fraction, Sr/Sr, and trace element geochemistry. We compared spatial patterns in metal flux and abundance with community-level socioeconomic metrics. We observed the highest dust fluxes at sites near the GSL playa. Within the urban corridor, Sr/Sr and trace element relative abundances suggest that most of the dust to which people are regularly exposed may be fugitive dust from local soil materials. The trace metal content of dust deposited along the Wasatch Front exceeded Environmental Protection Agency screening levels and exhibited enrichment relative to both the upper continental crust and the dust collected adjacent to GSL. Sources of metals to dust deposited along the Wasatch Front may include industrial activities like mining, oil refining, as well as past historical pesticide and herbicide applications. Arsenic and vanadium indicated a statistically significant positive correlation with income, whereas lead, thallium, and nickel exhibited higher concentrations in the least wealthy and least white neighborhoods.
美国犹他州的盐湖谷靠近干涸的大盐湖(GSL)。先前的研究发现,这个湖床/干盐湖会将富含金属的尘埃输送到瓦萨奇山脉和尤因塔山脉的雪中。尘埃和工业颗粒物污染也会输送到瓦萨奇山前的社区,但其来源、成分和通量特征尚不明确。在本研究中,我们分析了位于大盐湖附近、盐湖谷内及周边城市的18个被动采样器中沉积的尘埃,以测定总尘埃通量、<63 µm尘埃组分、锶同位素比值(Sr/Sr)以及微量元素地球化学特征。我们将金属通量和丰度的空间模式与社区层面的社会经济指标进行了比较。我们观察到在大盐湖干盐湖附近的采样点尘埃通量最高。在城市走廊内,Sr/Sr和微量元素相对丰度表明,人们经常接触到的大部分尘埃可能是来自当地土壤物质的扬尘。瓦萨奇山前沉积尘埃中的痕量金属含量超过了美国环境保护局的筛选水平,并且相对于上地壳和在大盐湖附近采集的尘埃都表现出富集。瓦萨奇山前沉积尘埃中的金属来源可能包括采矿、炼油等工业活动,以及过去使用过的农药和除草剂。砷和钒与收入呈统计学显著正相关,而铅、铊和镍在最贫困和白人比例最低的社区中浓度较高。