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基于金纳米岛的自参考折射率传感器。

A Self-Referenced Refractive Index Sensor Based on Gold Nanoislands.

机构信息

Department of Photonics and Bioengineering, CEMDATIC, ETSI Telecomunicación, Universidad Politécnica de Madrid, Ciudad Universitaria s/n, 28040 Madrid, Spain.

Department of Electronic Engineering, CEMDATIC, ETSI Telecomunicación, Universidad Politécnica de Madrid, Ciudad Universitaria s/n, 28040 Madrid, Spain.

出版信息

Sensors (Basel). 2022 Dec 21;23(1):66. doi: 10.3390/s23010066.

Abstract

We report on a self-referenced refractive index optical sensor based on Au nanoislands. The device consists of a random distribution of Au nanoislands formed by dewetting on a planar SiO/metal Fabry-Pérot cavity. Experimental and theoretical studies of the reflectance of this configuration reveal that its spectral response results from a combination of two resonances: a localized surface plasmon resonance (LSPR) associated to the Au nanoislands and the lowest-order anti-symmetric resonance of the Fabry-Pérot cavity. When the device is immersed in different fluids, the LSPR contribution provides high sensitivity to refractive index variations of the fluid, whereas those refractive index changes have little impact on the Fabry-Pérot resonance wavelength, allowing its use as a reference signal. The self-referenced sensor exhibits a spectral sensitivity of 212 nm/RIU (RIU: refractive index unit), which is larger than those of similar structures, and an intensity sensitivity of 4.9 RIU. The proposed chip-based architecture and the low cost and simplicity of the Au nanoisland synthesis procedure make the demonstrated sensor a promising self-referenced plasmonic sensor for compact biosensing optical platforms based on reflection mode operation.

摘要

我们报告了一种基于金纳米岛的自参考折射率光学传感器。该器件由在平面 SiO/金属法布里-珀罗腔上进行去湿形成的随机分布的金纳米岛组成。对该结构反射率的实验和理论研究表明,其光谱响应是由两个共振的组合产生的:与金纳米岛相关的局域表面等离子体共振(LSPR)和法布里-珀罗腔的最低阶反对称共振。当器件浸入不同的流体中时,LSPR 贡献对流体的折射率变化具有高灵敏度,而这些折射率变化对法布里-珀罗共振波长几乎没有影响,允许将其用作参考信号。自参考传感器表现出 212nm/RIU(RIU:折射率单位)的光谱灵敏度,大于类似结构的灵敏度,并且强度灵敏度为 4.9 RIU。所提出的基于芯片的架构以及金纳米岛合成过程的低成本和简单性使得所展示的传感器成为基于反射模式操作的紧凑型生物传感光学平台的有前途的自参考等离子体传感器。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/94d8/9824277/2cd45acae3ed/sensors-23-00066-g001.jpg

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