Ivanova Mariya E, Peters Ralf, Müller Martin, Haas Stefan, Seidler Martin Florian, Mutschke Gerd, Eckert Kerstin, Röse Philipp, Calnan Sonya, Bagacki Rory, Schlatmann Rutger, Grosselindemann Cedric, Schäfer Laura-Alena, Menzler Norbert H, Weber André, van de Krol Roel, Liang Feng, Abdi Fatwa F, Brendelberger Stefan, Neumann Nicole, Grobbel Johannes, Roeb Martin, Sattler Christian, Duran Ines, Dietrich Benjamin, Hofberger M E Christoph, Stoppel Leonid, Uhlenbruck Neele, Wetzel Thomas, Rauner David, Hecimovic Ante, Fantz Ursel, Kulyk Nadiia, Harting Jens, Guillon Olivier
Institute of Energy and Climate Research IEK-1: Materials Synthesis and Processing, Forschungszentrum Jülich GmbH (FZJ), Leo-Brandt-Str., 52425, Jülich, Germany.
Institute of Energy and Climate Research IEK-14: Electrochemical Process Engineering, Forschungszentrum Jülich GmbH (FZJ), Leo-Brandt-Str., 52425, Jülich, Germany.
Angew Chem Int Ed Engl. 2023 Aug 7;62(32):e202218850. doi: 10.1002/anie.202218850. Epub 2023 May 9.
Hydrogen (H ) produced from renewables will have a growing impact on the global energy dynamics towards sustainable and carbon-neutral standards. The share of green H is still too low to meet the net-zero target, while the demand for high-quality hydrogen continues to rise. These factors amplify the need for economically viable H generation technologies. The present article aims at evaluating the existing technologies for high-quality H production based on solar energy. Technologies such as water electrolysis, photoelectrochemical and solar thermochemical water splitting, liquid metal reactors and plasma conversion utilize solar power directly or indirectly (as carbon-neutral electrons) and are reviewed from the perspective of their current development level, technical limitations and future potential.
可再生能源制氢（H₂）将对全球能源动态朝着可持续和碳中和标准发展产生越来越大的影响。绿色氢气的占比仍过低，无法实现净零目标，而对高质量氢气的需求却持续上升。这些因素凸显了对经济可行的制氢技术的需求。本文旨在评估基于太阳能生产高质量氢气的现有技术。诸如水电解、光电化学和太阳能热化学水分解、液态金属反应堆以及等离子体转化等技术直接或间接利用太阳能（作为碳中和电子），并从其当前发展水平、技术局限性和未来潜力的角度进行了综述。
