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油气甲烷排放的起源:空中测量源的现场调查。

Origins of Oil and Gas Sector Methane Emissions: On-Site Investigations of Aerial Measured Sources.

机构信息

Energy & Emissions Research Laboratory, Department of Mechanical and Aerospace Engineering, Carleton University, Ottawa, Ontario K1S 5B6, Canada.

出版信息

Environ Sci Technol. 2023 Feb 14;57(6):2484-2494. doi: 10.1021/acs.est.2c07318. Epub 2023 Jan 30.

Abstract

Success in reducing oil and gas sector methane emissions is contingent on understanding the sources driving emissions, associated options for mitigation, and the effectiveness of regulations in achieving intended outcomes. This study combines high-resolution, high-sensitivity aerial survey data with subsequent on-site investigations of detected sources to examine these points. Measurements were performed in British Columbia, Canada, an active oil- and gas-producing province with modern methane regulations featuring mandatory three times per year leak detection and repair (LDAR) surveys at most facilities. Derived emission factors enabled by source attribution show that significant methane emissions persist under this regulatory framework, dominated by (i) combustion slip (compressor exhaust and also catalytic heaters, which are not covered in current regulations), (ii) intentional venting (uncontrolled tanks, vent stacks or intentionally unlit flares, and uncontrolled compressors), and (iii) unintentional venting (controlled tanks, unintentionally unlit/blown out flares, and abnormally operating pneumatics). Although the detailed analysis shows mitigation options exist for all sources, the importance of combustion slip and the persistently large methane contributions from controlled tanks and unlit flares demonstrate the limits of current LDAR programs and the critical need for additional monitoring and verification if regulations are to have the intended impacts, and reduction targets of 75% and greater are to be met.

摘要

成功减少油气行业甲烷排放取决于理解驱动排放的源头、相关减排选项,以及法规在实现预期目标方面的有效性。本研究结合了高分辨率、高灵敏度的航空调查数据以及随后对已检测到的排放源的现场调查,来研究这些问题。该研究在加拿大不列颠哥伦比亚省进行,这是一个活跃的产油和产气省份,其现代甲烷法规要求大多数设施每年进行三次强制性的泄漏检测和修复 (LDAR) 调查。通过源归因得出的排放因子表明,在这种监管框架下,仍存在大量甲烷排放,主要由(i)燃烧泄漏(压缩机废气,以及当前法规未涵盖的催化加热器)、(ii)故意放空(无控制的储罐、放空烟囱或故意未点燃的火炬以及无控制的压缩机)和(iii)意外放空(有控制的储罐、意外未点燃/吹灭的火炬以及非正常运行的气动装置)造成。尽管详细分析表明所有排放源都存在减排选项,但燃烧泄漏的重要性以及有控制的储罐和未点燃的火炬持续大量排放甲烷,表明当前 LDAR 计划存在局限性,如果要实现法规的预期影响,以及要达到 75%及以上的减排目标,就需要额外的监测和验证。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/dfc6/9933527/bc26ce85fe61/es2c07318_0002.jpg

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