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基于二碲化钼/二硫化钼异质结构的应变不敏感柔性光电探测器。

Strain insensitive flexible photodetector based on molybdenum ditelluride/molybdenum disulfide heterostructure.

作者信息

Zhu Xuesong, Wu Dahao, Liang Shengzhi, Liu Jing

机构信息

State Key Laboratory of Precision Measurement Technology and Instrument, School of Precision Instruments and Opto-electronics Engineering, Tianjin University, No. 92 Weijin Road, Tianjin, 300072, People's Republic of China.

出版信息

Nanotechnology. 2023 Feb 3;34(15). doi: 10.1088/1361-6528/acb359.

Abstract

Flexible electronic and optoelectronic devices are highly desirable for various emerging applications, such as human-computer interfaces, wearable medical electronics, flexible display, etc. Layered two-dimensional (2D) material is one of the most promising types of materials to develop flexible devices due to its atomically thin thickness, which gives it excellent flexibility and mechanical endurance. However, the 2D material devices fabricated on flexible substrate inevitably suffer from mechanical deformation, which can severely affect device performances, resulting in function degradation and even failure. In this work, we propose a strain insensitive flexible photodetector based on MoS/MoTeheterostructure on polyimide substrate, which provides a feasible approach to cancel unpredicted impacts of strain on the device performances. Specifically, the MoS/MoTeheterostructure is deposited with 4 electrodes to form three independent devices of MoSFET, MoTeFET and MoS/MoTeheterojunction. Among them, the MoS/MoTeheterojunction is used as the photodetector, while the MoSFET is used as a strain gauge to calibrate the photo detection result. Such configuration is enabled by the Schottky barrier formed between the electrodes and the MoSflake, which leads to obvious and negligible photo response of MoS/MoTeheterojunction and MoSFET, respectively, under low source-drain bias (ex. 10 mV). The experimental results show that the proposed mechanism can not only calibrate the photo response to cancel strain effect, but also successfully differentiate the wavelength (with fixed power) or power (with fixed wavelength) of light illumination.

摘要

柔性电子和光电器件对于各种新兴应用来说是非常理想的,比如人机接口、可穿戴医疗电子设备、柔性显示器等。层状二维(2D)材料是开发柔性器件最有前景的材料类型之一,因为其原子级的超薄厚度赋予了它出色的柔韧性和机械耐久性。然而,在柔性基板上制造的二维材料器件不可避免地会受到机械变形的影响,这会严重影响器件性能,导致功能退化甚至失效。在这项工作中,我们提出了一种基于聚酰亚胺基板上的MoS/MoTe异质结构的应变不敏感柔性光电探测器,它提供了一种可行的方法来消除应变对器件性能的不可预测影响。具体来说,MoS/MoTe异质结构沉积有4个电极,形成了MoSFET、MoTeFET和MoS/MoTe异质结三个独立的器件。其中,MoS/MoTe异质结用作光电探测器,而MoSFET用作应变计来校准光检测结果。这种配置是由电极和MoS薄片之间形成的肖特基势垒实现的,这导致在低源漏偏压(例如10 mV)下,MoS/MoTe异质结和MoSFET分别具有明显且可忽略的光响应。实验结果表明,所提出的机制不仅可以校准光响应以消除应变效应,还能成功区分光照的波长(固定功率)或功率(固定波长)。

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