Kroychuk Maria K, Shorokhov Alexander S, Yagudin Damir F, Rakhlin Maxim V, Klimko Grigorii V, Toropov Alexey A, Shubina Tatiana V, Fedyanin Andrey A
Faculty of Physics, Lomonosov Moscow State University, 119991 Moscow, Russia.
Ioffe Institute, 194021 St. Petersburg, Russia.
Nanomaterials (Basel). 2023 Jan 27;13(3):507. doi: 10.3390/nano13030507.
Single photon sources based on semiconductor quantum dots are one of the most prospective elements for optical quantum computing and cryptography. Such systems are often based on Bragg resonators, which provide several ways to control the emission of quantum dots. However, the fabrication of periodic structures with many thin layers is difficult. On the other hand, the coupling of single-photon sources with resonant nanoclusters made of high-index dielectric materials is known as a promising way for emission control. Our experiments and calculations show that the excitation of magnetic Mie-type resonance by linearly polarized light in a GaAs nanopillar oligomer with embedded InAs quantum dots leads to quantum emitters absorption efficiency enhancement. Moreover, the nanoresonator at the wavelength of magnetic dipole resonance also acts as a nanoantenna for a generated signal, allowing control over its radiation spatial profile. We experimentally demonstrated an order of magnitude emission enhancement and numerically reached forty times gain in comparison with unstructured film. These findings highlight the potential of quantum dots coupling with Mie-resonant oligomers collective modes for nanoscale single-photon sources development.
基于半导体量子点的单光子源是光学量子计算和密码学中最具前景的元素之一。此类系统通常基于布拉格谐振器,它提供了多种控制量子点发射的方法。然而,制造具有许多薄层的周期性结构很困难。另一方面,单光子源与由高折射率介电材料制成的共振纳米团簇的耦合是一种很有前景的发射控制方法。我们的实验和计算表明,在嵌入了砷化铟量子点的砷化镓纳米柱低聚物中,线偏振光激发磁米氏型共振会导致量子发射器吸收效率提高。此外,磁偶极子共振波长处的纳米谐振器还充当所产生信号的纳米天线,从而可以控制其辐射空间分布。与非结构化薄膜相比,我们通过实验证明了发射增强了一个数量级,通过数值计算实现了四十倍的增益。这些发现突出了量子点与米氏共振低聚物集体模式耦合在纳米级单光子源开发中的潜力。