Kang Yifan, Yang Hongtao, Wang Chao, Li Yongfeng, Xu Peng
Xi'an Institute of Optics and Precision Mechanics of Chinese Academy of Sciences, Xi'an 710119, China.
University of Chinese Academy of Sciences, Beijing 100049, China.
Heliyon. 2023 Jan 20;9(2):e13084. doi: 10.1016/j.heliyon.2023.e13084. eCollection 2023 Feb.
Based on a petal-like microstructure model of alloy particles we proposed, the field-regulating characteristics of alloy-based metamaterial films in the wavelength range of 300-800 nm are analyzed. It is found that Au/Ag alloy particles can support a broader resonance band with higher averaged resonance intensities than that of pure silver or gold particles, which, named alloy plasmonic effect, proves to be a universal feature of alloy-based plasmonics. Upon optimizing the coupling interaction between the alloy plasmonic effect and absorption saturation effect within alloy-based multilaminar structures, a broadband electromagnetic wave absorber consisting of a Cu/Al alloy-based composites layer and an aluminum base layer is demonstrated. Furthermore, a generalized method is proposed to evaluate the absorption performance of this kind of plasmonic absorber. The achieved alloy-based absorber proves to be nearly non-iridescent and the quality factor AP throughout the range of 300-800 nm remains higher than 0.8 even if the incident angle increases up to 60°.
基于我们提出的合金颗粒花瓣状微观结构模型,分析了合金基超材料薄膜在300 - 800纳米波长范围内的场调控特性。研究发现,与纯银或金颗粒相比,金/银合金颗粒能支持更宽的共振带且平均共振强度更高,这种现象被称为合金等离子体效应,是合金基等离子体学的一个普遍特征。通过优化合金基多层结构中合金等离子体效应与吸收饱和效应之间的耦合相互作用,展示了一种由铜/铝合金基复合材料层和铝基层组成的宽带电磁波吸收器。此外,还提出了一种通用方法来评估这种等离子体吸收器的吸收性能。所制备的合金基吸收器几乎无虹彩现象,即使入射角增大到60°,在300 - 800纳米范围内的品质因数AP仍高于0.8。