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太赫兹互相关光谱学与大面积石墨烯成像

Terahertz Cross-Correlation Spectroscopy and Imaging of Large-Area Graphene.

机构信息

Department of Electrical and Photonics Engineering, Technical University of Denmark, 2800 Kongens Lyngby, Denmark.

GLAZE Technologies Aps, 2950 Vedbæk, Denmark.

出版信息

Sensors (Basel). 2023 Mar 21;23(6):3297. doi: 10.3390/s23063297.

DOI:10.3390/s23063297
PMID:36992008
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10059862/
Abstract

We demonstrate the use of a novel, integrated THz system to obtain time-domain signals for spectroscopy in the 0.1-1.4 THz range. The system employs THz generation in a photomixing antenna excited by a broadband amplified spontaneous emission (ASE) light source and THz detection with a photoconductive antenna by coherent cross-correlation sampling. We benchmark the performance of our system against a state-of-the-art femtosecond-based THz time-domain spectroscopy system in terms of mapping and imaging of the sheet conductivity of large-area graphene grown by chemical vapor deposition (CVD) and transferred to a PET polymer substrate. We propose to integrate the algorithm for the extraction of the sheet conductivity with the data acquisition, thereby enabling true in-line monitoring capability of the system for integration in graphene production facilities.

摘要

我们展示了一种新颖的集成太赫兹系统的应用,该系统可用于在 0.1-1.4 太赫兹范围内获得光谱时域信号。该系统采用在宽带放大自发辐射(ASE)光源激发下的光电混合天线产生太赫兹波,并通过相干互相关采样的光电导天线进行太赫兹探测。我们将我们的系统与基于飞秒的太赫兹时域光谱系统的性能进行了基准测试,比较了它们在大面积化学气相沉积(CVD)生长并转移到 PET 聚合物衬底上的石墨烯的面电导率的测绘和成像方面的性能。我们提出将面电导率提取算法与数据采集集成在一起,从而为系统提供真正的在线监测能力,以便集成到石墨烯生产设备中。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/aa9c644951b8/sensors-23-03297-g011.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/065b1f41e0a4/sensors-23-03297-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/9b093fc223a0/sensors-23-03297-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/59b1381f75ff/sensors-23-03297-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/d721bacd745e/sensors-23-03297-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/b70607624d04/sensors-23-03297-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/7d216742b6fd/sensors-23-03297-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/d912e798b942/sensors-23-03297-g007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/2ce33c335f58/sensors-23-03297-g008.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/e9e212ee1326/sensors-23-03297-g009.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/20d65fd22a9a/sensors-23-03297-g010.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/aa9c644951b8/sensors-23-03297-g011.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/065b1f41e0a4/sensors-23-03297-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/9b093fc223a0/sensors-23-03297-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/59b1381f75ff/sensors-23-03297-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/d721bacd745e/sensors-23-03297-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/b70607624d04/sensors-23-03297-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/7d216742b6fd/sensors-23-03297-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/d912e798b942/sensors-23-03297-g007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/2ce33c335f58/sensors-23-03297-g008.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/e9e212ee1326/sensors-23-03297-g009.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/20d65fd22a9a/sensors-23-03297-g010.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1797/10059862/aa9c644951b8/sensors-23-03297-g011.jpg

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引用本文的文献

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Correction: Mølvig et al. Terahertz Cross-Correlation Spectroscopy and Imaging of Large-Area Graphene. 2023, , 3297.更正:莫尔维格等人。大面积石墨烯的太赫兹互相关光谱学与成像。2023年,,3297。 (注:原文中存在格式上的不规范,如两个逗号,翻译时保留了原文的格式问题)
Sensors (Basel). 2025 Jun 23;25(13):3895. doi: 10.3390/s25133895.
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A Hardware Encoder-Based Synchronization Method for a Fast Terahertz TDS Imaging System Based on the ECOPS Scheme.一种基于硬件编码器的、用于基于ECOPS方案的快速太赫兹时域光谱成像系统的同步方法。
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Strain versus Tunable Terahertz Nanogap Width: A Simple Formula and a Trench below.

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