Department of Physics, Harvard University, Cambridge, MA, 02138, USA.
Department of Physics and Astronomy, Purdue University, West Lafayette, IN, 47907, USA.
Nat Commun. 2023 May 5;14(1):2622. doi: 10.1038/s41467-023-38249-3.
Charge modulations have been widely observed in cuprates, suggesting their centrality for understanding the high-T superconductivity in these materials. However, the dimensionality of these modulations remains controversial, including whether their wavevector is unidirectional or bidirectional, and also whether they extend seamlessly from the surface of the material into the bulk. Material disorder presents severe challenges to understanding the charge modulations through bulk scattering techniques. We use a local technique, scanning tunneling microscopy, to image the static charge modulations on BiPbSrLaCuO. The ratio of the phase correlation length ξ to the orientation correlation length ξ points to unidirectional charge modulations. By computing new critical exponents at free surfaces including that of the pair connectivity correlation function, we show that these locally 1D charge modulations are actually a bulk effect resulting from classical 3D criticality of the random field Ising model throughout the entire superconducting doping range.
电荷调制在铜氧化物中被广泛观察到,这表明它们对于理解这些材料中的高温超导性至关重要。然而,这些调制的维度仍然存在争议,包括其波矢是单向的还是双向的,以及它们是否从材料表面无缝地延伸到体相。材料无序给通过体散射技术理解电荷调制带来了严峻的挑战。我们使用一种局部技术,扫描隧道显微镜,来成像 BiPbSrLaCuO 上的静态电荷调制。相位相关长度 ξ 与方向相关长度 ξ 之比指向单向电荷调制。通过计算包括对关联函数在内的自由表面的新临界指数,我们表明这些局域的一维电荷调制实际上是体相效应,是整个超导掺杂范围内随机场伊辛模型的经典三维临界性的结果。