Putri Linda Ardita, Rahman Iman, Puspita Mayumi, Hidayat Shidiq Nur, Dharmawan Agus Budi, Rianjanu Aditya, Wibirama Sunu, Roto Roto, Triyana Kuwat, Wasisto Hutomo Suryo
PT Nanosense Instrument Indonesia, Yogyakarta, 55167, Indonesia.
Department of Physics, Faculty of Mathematics and Natural Sciences, Universitas Gadjah Mada, Sekip Utara PO Box BLS 21, Yogyakarta, 55281, Indonesia.
NPJ Sci Food. 2023 Jun 16;7(1):31. doi: 10.1038/s41538-023-00205-2.
Authentication of meat floss origin has been highly critical for its consumers due to existing potential risks of having allergic diseases or religion perspective related to pork-containing foods. Herein, we developed and assessed a compact portable electronic nose (e-nose) comprising gas sensor array and supervised machine learning with a window time slicing method to sniff and to classify different meat floss products. We evaluated four different supervised learning methods for data classification (i.e., linear discriminant analysis (LDA), quadratic discriminant analysis (QDA), k-nearest neighbors (k-NN), and random forest (RF)). Among them, an LDA model equipped with five-window-extracted feature yielded the highest accuracy values of >99% for both validation and testing data in discriminating beef, chicken, and pork flosses. The obtained e-nose results were correlated and confirmed with the spectral data from Fourier-transform infrared (FTIR) spectroscopy and gas chromatography-mass spectrometry (GC-MS) measurements. We found that beef and chicken had similar compound groups (i.e., hydrocarbons and alcohol). Meanwhile, aldehyde compounds (e.g., dodecanal and 9-octadecanal) were found to be dominant in pork products. Based on its performance evaluation, the developed e-nose system shows promising results in food authenticity testing, which paves the way for ubiquitously detecting deception and food fraud attempts.
由于食用含猪肉食品存在过敏疾病或宗教方面的潜在风险,肉松来源的鉴定对消费者来说至关重要。在此,我们开发并评估了一种紧凑型便携式电子鼻,它由气体传感器阵列和采用窗口时间切片方法的监督机器学习组成,用于嗅探和分类不同的肉松产品。我们评估了四种不同的监督学习方法用于数据分类(即线性判别分析(LDA)、二次判别分析(QDA)、k近邻(k-NN)和随机森林(RF))。其中,配备五个窗口提取特征的LDA模型在区分牛肉、鸡肉和猪肉松的验证数据和测试数据方面均产生了高于99%的最高准确率值。获得的电子鼻结果与傅里叶变换红外(FTIR)光谱和气相色谱-质谱(GC-MS)测量的光谱数据相关且得到了证实。我们发现牛肉和鸡肉具有相似的化合物组(即碳氢化合物和醇类)。同时,醛类化合物(如十二醛和9-十八醛)在猪肉产品中占主导地位。基于其性能评估,所开发的电子鼻系统在食品真实性检测方面显示出有前景的结果,这为普遍检测欺诈和食品掺假企图铺平了道路。