Attwood Max, Xu Xiaotian, Newns Michael, Meng Zhu, Ingle Rebecca A, Wu Hao, Chen Xi, Xu Weidong, Ng Wern, Abiola Temitope T, Stavros Vasilios G, Oxborrow Mark
Department of Materials, Imperial College London, South Kensington Campus, Exhibition Road, London SW7 2AZ, U.K.
Molecular Sciences Research Hub, Department of Chemistry, Imperial College London, White City Campus, 82 Wood Lane, London W12 0BZ, U.K.
Chem Mater. 2023 May 23;35(11):4498-4509. doi: 10.1021/acs.chemmater.3c00640. eCollection 2023 Jun 13.
The development of future quantum devices such as the maser, i.e., the microwave analog of the laser, could be well-served by the exploration of chemically tunable organic materials. Current iterations of room-temperature organic solid-state masers are composed of an inert host material that is doped with a spin-active molecule. In this work, we systematically modulated the structure of three nitrogen-substituted tetracene derivatives to augment their photoexcited spin dynamics and then evaluated their potential as novel maser gain media by optical, computational, and electronic paramagnetic resonance (EPR) spectroscopy. To facilitate these investigations, we adopted an organic glass former, 1,3,5-tri(1-naphthyl)benzene to act as a universal host. These chemical modifications impacted the rates of intersystem crossing, triplet spin polarization, triplet decay, and spin-lattice relaxation, leading to significant consequences on the conditions required to surpass the maser threshold.
诸如微波激射器(即激光的微波类似物)等未来量子器件的发展,可以通过探索化学可调谐有机材料得到很好的推动。室温有机固态微波激射器的当前迭代版本由掺杂有自旋活性分子的惰性主体材料组成。在这项工作中,我们系统地调制了三种氮取代并四苯衍生物的结构,以增强其光激发自旋动力学,然后通过光学、计算和电子顺磁共振(EPR)光谱评估它们作为新型微波激射增益介质的潜力。为便于进行这些研究,我们采用了一种有机玻璃形成剂1,3,5-三(1-萘基)苯作为通用主体。这些化学修饰影响了系间窜越速率、三重态自旋极化、三重态衰减和自旋晶格弛豫,对超过微波激射阈值所需的条件产生了重大影响。