Department of Quantum Matter Physics, University of Geneva, 1211, Geneva, Switzerland.
Department of Theoretical Physics, University of Geneva, 1211, Geneva, Switzerland.
Nat Commun. 2023 Jun 24;14(1):3771. doi: 10.1038/s41467-023-39453-x.
Inducing and controlling spin-orbit coupling (SOC) in graphene is key to create topological states of matter, and for the realization of spintronic devices. Placing graphene onto a transition metal dichalcogenide is currently the most successful strategy to achieve this goal, but there is no consensus as to the nature and the magnitude of the induced SOC. Here, we show that the presence of backscattering in graphene-on-WSe heterostructures can be used to probe SOC and to determine its strength quantitatively, by imaging quasiparticle interference with a scanning tunneling microscope. A detailed theoretical analysis of the Fourier transform of quasiparticle interference images reveals that the induced SOC consists of a valley-Zeeman (λ ≈ 2 meV) and a Rashba (λ ≈ 15 meV) term, one order of magnitude larger than what theory predicts, but in excellent agreement with earlier transport experiments. The validity of our analysis is confirmed by measurements on a 30 degree twist angle heterostructure that exhibits no backscattering, as expected from symmetry considerations. Our results demonstrate a viable strategy to determine SOC quantitatively by imaging quasiparticle interference.
在石墨烯中诱导和控制自旋轨道耦合(SOC)是创造物质拓扑状态和实现自旋电子器件的关键。将石墨烯置于过渡金属二卤化物上是目前实现这一目标最成功的策略,但对于所诱导的 SOC 的性质和大小还没有共识。在这里,我们通过扫描隧道显微镜成像来探测 SOC 并定量确定其强度,展示了在石墨烯/ WSe 异质结构中存在背散射可以用于探测 SOC。对准粒子干涉的傅里叶变换的详细理论分析表明,所诱导的 SOC 由谷-塞曼(λ≈2meV)和拉什巴(λ≈15meV)项组成,其量级比理论预测的大一个数量级,但与早期的输运实验非常吻合。通过对预期从对称性考虑不会发生背散射的 30 度扭转角异质结构的测量,证实了我们分析的有效性。我们的结果展示了一种通过成像准粒子干涉来定量确定 SOC 的可行策略。