Del Águila Andrés Granados, Wong Yi Ren, Wadgaonkar Indrajit, Fieramosca Antonio, Liu Xue, Vaklinova Kristina, Dal Forno Stefano, Do T Thu Ha, Wei Ho Yi, Watanabe K, Taniguchi T, Novoselov Kostya S, Koperski Maciej, Battiato Marco, Xiong Qihua
Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore, Singapore.
Institutes of Physical Science and Information Technology, Anhui University, Hefei, P.R. China.
Nat Nanotechnol. 2023 Sep;18(9):1012-1019. doi: 10.1038/s41565-023-01438-8. Epub 2023 Jul 31.
Excitons (coupled electron-hole pairs) in semiconductors can form collective states that sometimes exhibit spectacular nonlinear properties. Here, we show experimental evidence of a collective state of short-lived excitons in a direct-bandgap, atomically thin MoS semiconductor whose propagation resembles that of a classical liquid as suggested by the nearly uniform photoluminescence through the MoS monolayer regardless of crystallographic defects and geometric constraints. The exciton fluid flows over ultralong distances (at least 60 μm) at a speed of 1.8 × 10 m s (6% the speed of light). The collective phase emerges above a critical laser power, in the absence of free charges and below a critical temperature (usually T ≈ 150 K) approaching room temperature in hexagonal-boron-nitride-encapsulated devices. Our theoretical simulations suggest that momentum is conserved and local equilibrium is achieved among excitons; both these features are compatible with a fluid dynamics description of the exciton transport.
半导体中的激子(耦合的电子 - 空穴对)可以形成集体态,这些集体态有时会表现出惊人的非线性特性。在此,我们展示了在直接带隙、原子级薄的二硫化钼(MoS)半导体中短寿命激子集体态的实验证据,其传播类似于经典液体,这是由通过MoS单层的几乎均匀的光致发光所表明的,而与晶体缺陷和几何约束无关。激子流体以约1.8×10⁵m/s(约为光速的6%)的速度在超长距离(至少60μm)上流动。在临界激光功率以上、没有自由电荷且在临界温度以下(在六方氮化硼封装的器件中,临界温度通常T≈150K)接近室温时,集体相出现。我们的理论模拟表明,激子之间动量守恒且达到局部平衡;这两个特征都与激子输运的流体动力学描述相一致。