Yoon Ju-Young, Zhang Pengxiang, Chou Chung-Tao, Takeuchi Yutaro, Uchimura Tomohiro, Hou Justin T, Han Jiahao, Kanai Shun, Ohno Hideo, Fukami Shunsuke, Liu Luqiao
Laboratory for Nanoelectronics and Spintronics, Research Institute of Electrical Communication, Tohoku University, Sendai, Japan.
Graduate School of Engineering, Tohoku University, Sendai, Japan.
Nat Mater. 2023 Sep;22(9):1106-1113. doi: 10.1038/s41563-023-01620-2. Epub 2023 Aug 3.
Non-collinear antiferromagnets are an emerging family of spintronic materials because they not only possess the general advantages of antiferromagnets but also enable more advanced functionalities. Recently, in an intriguing non-collinear antiferromagnet MnSn, where the octupole moment is defined as the collective magnetic order parameter, spin-orbit torque (SOT) switching has been achieved in seemingly the same protocol as in ferromagnets. Nevertheless, it is fundamentally important to explore the unknown octupole moment dynamics and contrast it with the magnetization vector of ferromagnets. Here we report a handedness anomaly in the SOT-driven dynamics of MnSn: when spin current is injected, the octupole moment rotates in the opposite direction to the individual moments, leading to a SOT switching polarity distinct from ferromagnets. By using second-harmonic and d.c. magnetometry, we track the SOT effect onto the octupole moment during its rotation and reveal that the handedness anomaly stems from the interactions between the injected spin and the unique chiral-spin structure of MnSn. We further establish the torque balancing equation of the magnetic octupole moment and quantify the SOT efficiency. Our finding provides a guideline for understanding and implementing the electrical manipulation of non-collinear antiferromagnets, which in nature differs from the well-established collinear magnets.
非共线反铁磁体是一类新兴的自旋电子材料,因为它们不仅具有反铁磁体的一般优点,还能实现更先进的功能。最近,在一种有趣的非共线反铁磁体MnSn中,八极矩被定义为集体磁有序参数,自旋轨道矩(SOT)开关似乎以与铁磁体相同的方式实现。然而,探索未知的八极矩动力学并将其与铁磁体的磁化矢量进行对比,在根本上具有重要意义。在此,我们报告了MnSn中SOT驱动动力学的手性异常:当注入自旋电流时,八极矩的旋转方向与单个磁矩相反,导致SOT开关极性与铁磁体不同。通过使用二次谐波和直流磁力测量,我们在八极矩旋转过程中追踪SOT对其的影响,并揭示出手性异常源于注入的自旋与MnSn独特的手性自旋结构之间的相互作用。我们进一步建立了磁八极矩的转矩平衡方程,并量化了SOT效率。我们的发现为理解和实现非共线反铁磁体的电操纵提供了指导,非共线反铁磁体本质上不同于已充分研究的共线磁体。