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Identification, Quantification, and Elimination of NO and NH Impurities for Aqueous and Li-Mediated Nitrogen Reduction Experiments.

作者信息

Izelaar Boaz, Ripepi Davide, van Noordenne Dylan D, Jungbacker Peter, Kortlever Ruud, Mulder Fokko M

机构信息

Large Scale Energy Storage, Process and Energy Department, Faculty of Mechanical, Maritime and Materials Engineering, Delft University of Technology, 2628 CB Delft, The Netherlands.

Materials for Energy Conversion and Storage, Chemical Engineering Department, Faculty of Applied Sciences, Delft University of Technology, 2629 HZ Delft, The Netherlands.

出版信息

ACS Energy Lett. 2023 Aug 2;8(8):3614-3620. doi: 10.1021/acsenergylett.3c01130. eCollection 2023 Aug 11.

DOI:10.1021/acsenergylett.3c01130
PMID:37588017
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10425974/
Abstract
摘要
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/998f/10425974/47ed953c0464/nz3c01130_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/998f/10425974/0098930268b0/nz3c01130_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/998f/10425974/f98f3b3b69a6/nz3c01130_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/998f/10425974/6e3af4ad8c59/nz3c01130_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/998f/10425974/47ed953c0464/nz3c01130_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/998f/10425974/0098930268b0/nz3c01130_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/998f/10425974/f98f3b3b69a6/nz3c01130_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/998f/10425974/6e3af4ad8c59/nz3c01130_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/998f/10425974/47ed953c0464/nz3c01130_0004.jpg

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Electrosynthesis of ammonia with high selectivity and high rates via engineering of the solid-electrolyte interphase.通过固体电解质界面工程实现高选择性和高反应速率的氨电合成。
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Electroreduction of nitrogen with almost 100% current-to-ammonia efficiency.
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