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长程哈肯-施特罗布尔-赖内克模型中的反常扩散

Anomalous Diffusion in the Long-Range Haken-Strobl-Reineker Model.

作者信息

Catalano A G, Mattiotti F, Dubail J, Hagenmüller D, Prosen T, Franchini F, Pupillo G

机构信息

University of Strasbourg and CNRS, CESQ and ISIS (UMR 7006), aQCess, 67000 Strasbourg, France.

Institut Ruđer Bošković, Bijenička cesta 54, 10000 Zagreb, Croatia.

出版信息

Phys Rev Lett. 2023 Aug 4;131(5):053401. doi: 10.1103/PhysRevLett.131.053401.

Abstract

We analyze the propagation of excitons in a d-dimensional lattice with power-law hopping ∝1/r^{α} in the presence of dephasing, described by a generalized Haken-Strobl-Reineker model. We show that in the strong dephasing (quantum Zeno) regime the dynamics is described by a classical master equation for an exclusion process with long jumps. In this limit, we analytically compute the spatial distribution, whose shape changes at a critical value of the decay exponent α_{cr}=(d+2)/2. The exciton always diffuses anomalously: a superdiffusive motion is associated to a Lévy stable distribution with long-range algebraic tails for α≤α_{cr}, while for α>α_{cr} the distribution corresponds to a surprising mixed Gaussian profile with long-range algebraic tails, leading to the coexistence of short-range diffusion and long-range Lévy flights. In the many-exciton case, we demonstrate that, starting from a domain-wall exciton profile, algebraic tails appear in the distributions for any α, which affects thermalization: the longer the hopping range, the faster equilibrium is reached. Our results are directly relevant to experiments with cold trapped ions, Rydberg atoms, and supramolecular dye aggregates. They provide a way to realize an exclusion process with long jumps experimentally.

摘要

我们分析了在存在退相干的情况下,激子在具有幂律跳跃∝1/r^α的d维晶格中的传播,该过程由广义哈肯 - 施特罗布尔 - 赖内克模型描述。我们表明,在强退相干(量子芝诺) regime中,动力学由具有长跳的排除过程的经典主方程描述。在此极限下,我们解析计算了空间分布,其形状在衰减指数α_cr = (d + 2)/2的临界值处发生变化。激子总是异常扩散:对于α≤α_cr,超扩散运动与具有长程代数尾的列维稳定分布相关,而对于α>α_cr,分布对应于具有长程代数尾的令人惊讶的混合高斯分布,导致短程扩散和长程列维飞行共存。在多激子情况下,我们证明,从畴壁激子分布开始,对于任何α,代数尾都会出现在分布中,这会影响热化:跳跃范围越长,达到平衡的速度越快。我们的结果与冷俘获离子、里德堡原子和超分子染料聚集体的实验直接相关。它们提供了一种在实验中实现具有长跳的排除过程的方法。

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