Abdi Jafar, Mazloom Golshan, Hadavimoghaddam Fahimeh, Hemmati-Sarapardeh Abdolhossein, Esmaeili-Faraj Seyyed Hamid, Bolhasani Akbar, Karamian Soroush, Hosseini Shahin
Faculty of Chemical and Materials Engineering, Shahrood University of Technology, Shahrood, Iran.
Department of Chemical Engineering, Faculty of Engineering, University of Mazandaran, Babolsar, Iran.
Sci Rep. 2023 Aug 28;13(1):14081. doi: 10.1038/s41598-023-41273-4.
Light olefins, as the backbone of the chemical and petrochemical industries, are produced mainly via steam cracking route. Prediction the of effects of operating variables on the product yield distribution through the mechanistic approaches is complex and requires long time. While increasing in the industrial automation and the availability of the high throughput data, the machine learning approaches have gained much attention due to the simplicity and less required computational efforts. In this study, the potential capability of four powerful machine learning models, i.e., Multilayer perceptron (MLP) neural network, adaptive boosting-support vector regression (AdaBoost-SVR), recurrent neural network (RNN), and deep belief network (DBN) was investigated to predict the product distribution of an olefin plant in industrial scale. In this regard, an extensive data set including 1184 actual data points were gathered during four successive years under various practical conditions. 24 varying independent parameters, including flow rates of different feedstock, numbers of active furnaces, and coil outlet temperatures, were chosen as the input variables of the models and the outputs were the flow rates of the main products, i.e., pyrolysis gasoline, ethylene, and propylene. The accuracy of the models was assessed by different statistical techniques. Based on the obtained results, the RNN model accurately predicted the main product flow rates with average absolute percent relative error (AAPRE) and determination coefficient (R) values of 1.94% and 0.97, 1.29% and 0.99, 0.70% and 0.99 for pyrolysis gasoline, propylene, and ethylene, respectively. The influence of the various parameters on the products flow rate (estimated by the RNN model) was studied by the relevancy factor calculation. Accordingly, the number of furnaces in service and the flow rates of some feedstock had more positive impacts on the outputs. In addition, the effects of different operating conditions on the propylene/ethylene (P/E) ratio as a cracking severity factor were also discussed. This research proved that intelligent approaches, despite being simple and straightforward, can predict complex unit performance. Thus, they can be efficiently utilized to control and optimize different industrial-scale units.
轻质烯烃作为化工和石化行业的支柱,主要通过蒸汽裂解路线生产。通过机理方法预测操作变量对产品产率分布的影响很复杂,且需要很长时间。随着工业自动化程度的提高和高通量数据的可得性,机器学习方法因其简单性和较少的计算量而备受关注。在本研究中,研究了四种强大的机器学习模型,即多层感知器(MLP)神经网络、自适应增强支持向量回归(AdaBoost-SVR)、递归神经网络(RNN)和深度信念网络(DBN)预测工业规模烯烃装置产品分布的潜在能力。为此,在连续四年的各种实际条件下收集了一个包含1184个实际数据点的广泛数据集。选择24个不同的独立参数,包括不同原料的流量、运行炉的数量和盘管出口温度,作为模型的输入变量,输出为主要产品的流量,即热解汽油、乙烯和丙烯。通过不同的统计技术评估模型的准确性。根据所得结果,RNN模型分别以1.94%和0.97、1.29%和0.99、0.70%和0.99的平均绝对百分比相对误差(AAPRE)和决定系数(R)值准确预测了热解汽油、丙烯和乙烯的主要产品流量。通过相关性因子计算研究了各种参数对产品流量(由RNN模型估计)的影响。因此,运行炉的数量和一些原料的流量对输出有更积极的影响。此外,还讨论了不同操作条件对作为裂解 severity 因子的丙烯/乙烯(P/E)比的影响。本研究证明,智能方法尽管简单直接,但可以预测复杂的装置性能。因此,它们可以有效地用于控制和优化不同的工业规模装置。