Poelchen G, Hellwig J, Peters M, Usachov D Yu, Kliemt K, Laubschat C, Echenique P M, Chulkov E V, Krellner C, Parkin S S P, Vyalikh D V, Ernst A, Kummer K
European Synchrotron Radiation Facility, 71 Avenue des Martyrs, 38043, Grenoble, France.
Institut für Festkörper- und Materialphysik, Technische Universität Dresden, 01062, Dresden, Germany.
Nat Commun. 2023 Sep 5;14(1):5422. doi: 10.1038/s41467-023-40963-x.
Collective spin excitations in magnetically ordered crystals, called magnons or spin waves, can serve as carriers in novel spintronic devices with ultralow energy consumption. The generation of well-detectable spin flows requires long lifetimes of high-frequency magnons. In general, the lifetime of spin waves in a metal is substantially reduced due to a strong coupling of magnons to the Stoner continuum. This makes metals unattractive for use as components for magnonic devices. Here, we present the metallic antiferromagnet CeCoP, which exhibits long-living magnons even in the terahertz (THz) regime. For CeCoP, our first-principle calculations predict a suppression of low-energy spin-flip Stoner excitations, which is verified by resonant inelastic X-ray scattering measurements. By comparison to the isostructural compound LaCoP, we show how small structural changes can dramatically alter the electronic structure around the Fermi level leading to the classical picture of the strongly damped magnons intrinsic to metallic systems. Our results not only demonstrate that long-lived magnons in the THz regime can exist in bulk metallic systems, but they also open a path for an efficient search for metallic magnetic systems in which undamped THz magnons can be excited.
磁有序晶体中的集体自旋激发,即磁振子或自旋波,可以作为新型超低能耗自旋电子器件中的载流子。产生可良好检测的自旋流需要高频磁振子具有较长的寿命。一般来说,由于磁振子与斯托纳连续体的强耦合,金属中自旋波的寿命会大幅缩短。这使得金属作为磁振子器件的组件缺乏吸引力。在此,我们展示了金属反铁磁体CeCoP,即使在太赫兹(THz)频段,它也表现出寿命较长的磁振子。对于CeCoP,我们的第一性原理计算预测了低能自旋翻转斯托纳激发的抑制,这一点通过共振非弹性X射线散射测量得到了验证。通过与同结构化合物LaCoP进行比较,我们展示了微小的结构变化如何显著改变费米能级附近的电子结构,从而导致金属系统中磁振子强阻尼的经典图像。我们的结果不仅表明太赫兹频段寿命较长的磁振子可以存在于体金属系统中,而且还为有效寻找能够激发无阻尼太赫兹磁振子的金属磁性系统开辟了一条道路。