Blank T G H, Grishunin K A, Ivanov B A, Mashkovich E A, Afanasiev D, Kimel A V
Radboud University, Institute for Molecules and Materials, 6525 AJ Nijmegen, The Netherlands.
Institute of Magnetism, National Academy of Sciences and Ministry of Education and Science, 03142 Kiev, Ukraine.
Phys Rev Lett. 2023 Sep 1;131(9):096701. doi: 10.1103/PhysRevLett.131.096701.
Finding efficient and ultrafast ways to control antiferromagnets is believed to be instrumental in unlocking their potential for magnetic devices operating at THz frequencies. Still, it is challenged by the absence of net magnetization in the ground state. Here, we show that the magnetization emerging from a state of coherent spin precession in antiferromagnetic iron borate FeBO_{3} can be used to enable the nonlinear coupling of light to another, otherwise weakly susceptible, mode of spin precession. This nonlinear mechanism can facilitate conceptually new ways of controlling antiferromagnetism.
人们认为,找到有效且超快的方法来控制反铁磁体有助于挖掘它们在太赫兹频率下运行的磁性器件中的潜力。然而,由于基态不存在净磁化强度,这一目标面临挑战。在此,我们表明,反铁磁硼酸铁FeBO₃中相干自旋进动状态产生的磁化强度可用于实现光与另一种原本弱响应的自旋进动模式的非线性耦合。这种非线性机制能够推动控制反铁磁性的全新概念方法。