Zhang Zhenya, Kanega Minoru, Maruyama Kei, Kurihara Takayuki, Nakajima Makoto, Tachizaki Takehiro, Sato Masahiro, Kanemitsu Yoshihiko, Hirori Hideki
Institute for Chemical Research, Kyoto University, Uji, Japan.
Department of Physics, Chiba University, Chiba, Japan.
Nat Mater. 2025 Feb;24(2):219-225. doi: 10.1038/s41563-024-02034-4. Epub 2024 Oct 25.
Driving spin systems to states far from equilibrium is indispensable in investigations of functional nonlinearities of antiferromagnets for spintronics. So far, it has been shown that electric-field pulses in the spectral region from the visible to the terahertz range can be used to induce ultrafast switching between different spin states. Here we demonstrate that a multicycle terahertz magnetic-field pulse can be used to induce non-thermal spin switching in antiferromagnets. When a strong pulse is applied to SmErFeO, the magnetic order parameter is first driven away from the barrier between the two potential minima of this antiferromagnet and then, in the subsequent inertial motion towards the opposite direction, it crosses the barrier. Our analysis reveals that the initial motion is driven by a dynamical modification of the magnetic potential, and this modification is enhanced through coupling between the two magnon modes.
在自旋电子学中,将自旋系统驱动到远离平衡的状态对于研究反铁磁体的功能非线性至关重要。到目前为止,已经表明,从可见光到太赫兹范围的光谱区域中的电场脉冲可用于诱导不同自旋状态之间的超快切换。在此,我们证明多周期太赫兹磁场脉冲可用于在反铁磁体中诱导非热自旋切换。当向SmErFeO施加强脉冲时,磁序参量首先被驱动远离该反铁磁体两个势阱之间的势垒,然后在随后向相反方向的惯性运动中穿过该势垒。我们的分析表明,初始运动是由磁势的动态改变驱动的,并且这种改变通过两个磁振子模式之间的耦合而增强。