Nielsen Leonard C, Erhart Paul, Guizar-Sicairos Manuel, Liebi Marianne
Department of Physics, Chalmers University of Technology, Gothenburg, Sweden.
Paul Scherrer Institute (PSI), Villigen, Switzerland.
Acta Crystallogr A Found Adv. 2023 Nov 1;79(Pt 6):515-526. doi: 10.1107/S205327332300863X. Epub 2023 Oct 19.
The development of small-angle scattering tensor tomography has enabled the study of anisotropic nanostructures in a volume-resolved manner. It is of great value to have reconstruction methods that can handle many different nanostructural symmetries. For such a method to be employed by researchers from a wide range of backgrounds, it is crucial that its reliance on prior knowledge about the system is minimized, and that it is robust under various conditions. Here, a method is presented that employs band-limited spherical functions to enable the reconstruction of reciprocal-space maps of a wide variety of nanostructures. This method has been thoroughly tested and compared with existing methods in its ability to retrieve known reciprocal-space maps, as well as its robustness to changes in initial conditions, using both simulations and experimental data. It has also been evaluated for its computational performance. The anchoring of this method in a framework of integral geometry and linear algebra highlights its possibilities and limitations.
小角散射张量断层扫描技术的发展使得以体素分辨的方式研究各向异性纳米结构成为可能。拥有能够处理多种不同纳米结构对称性的重建方法具有重要价值。为了让来自广泛背景的研究人员采用这样一种方法,至关重要的是尽量减少其对系统先验知识的依赖,并且使其在各种条件下都具有鲁棒性。在此,提出了一种方法,该方法利用带限球面函数来重建各种纳米结构的倒易空间图。此方法已经过全面测试,并在使用模拟和实验数据检索已知倒易空间图的能力以及对初始条件变化的鲁棒性方面与现有方法进行了比较。还对其计算性能进行了评估。该方法在积分几何和线性代数框架中的定位突出了其可能性和局限性。