Regmi Sabin, Bin Elius Iftakhar, Sakhya Anup Pradhan, Jeff Dylan, Sprague Milo, Mondal Mazharul Islam, Jarrett Damani, Valadez Nathan, Agosto Alexis, Romanova Tetiana, Chu Jiun-Haw, Khondaker Saiful I, Ptok Andrzej, Kaczorowski Dariusz, Neupane Madhab
Department of Physics, University of Central Florida, Orlando, FL 32816 USA.
Present Address: Center for Quantum Actinide Science and Technology, Idaho National laboratory, Idaho Falls, ID 83415 USA.
Sci Rep. 2023 Oct 30;13(1):18618. doi: 10.1038/s41598-023-44851-8.
Charge density wave (CDW) ordering has been an important topic of study for a long time owing to its connection with other exotic phases such as superconductivity and magnetism. The [Formula: see text] (R = rare-earth elements) family of materials provides a fertile ground to study the dynamics of CDW in van der Waals layered materials, and the presence of magnetism in these materials allows to explore the interplay among CDW and long range magnetic ordering. Here, we have carried out a high-resolution angle-resolved photoemission spectroscopy (ARPES) study of a CDW material [Formula: see text], which is antiferromagnetic below [Formula: see text], along with thermodynamic, electrical transport, magnetic, and Raman measurements. Our ARPES data show a two-fold symmetric Fermi surface with both gapped and ungapped regions indicative of the partial nesting. The gap is momentum dependent, maximum along [Formula: see text] and gradually decreases going towards [Formula: see text]. Our study provides a platform to study the dynamics of CDW and its interaction with other physical orders in two- and three-dimensions.
电荷密度波(CDW)有序化长期以来一直是一个重要的研究课题,因为它与超导和磁性等其他奇异相有关。[化学式:见正文](R = 稀土元素)材料家族为研究范德华层状材料中CDW的动力学提供了丰富的研究对象,并且这些材料中磁性的存在使得人们能够探索CDW与长程磁有序之间的相互作用。在此,我们对一种CDW材料[化学式:见正文]进行了高分辨率角分辨光电子能谱(ARPES)研究,该材料在[化学式:见正文]以下是反铁磁性的,同时还进行了热力学、电输运、磁性和拉曼测量。我们的ARPES数据显示出一个具有能隙和无能隙区域的二重对称费米面,这表明存在部分嵌套。能隙与动量有关,沿[化学式:见正文]方向最大,并朝着[化学式:见正文]方向逐渐减小。我们的研究提供了一个平台,用于研究二维和三维中CDW的动力学及其与其他物理有序态的相互作用。