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在电荷有序双层 Kagome 材料 ScVSn 中发现隐藏磁性。

Hidden magnetism uncovered in a charge ordered bilayer kagome material ScVSn.

作者信息

Guguchia Z, Gawryluk D J, Shin S, Hao Z, Mielke Iii C, Das D, Plokhikh I, Liborio L, Shenton J Kane, Hu Y, Sazgari V, Medarde M, Deng H, Cai Y, Chen C, Jiang Y, Amato A, Shi M, Hasan M Z, Yin J-X, Khasanov R, Pomjakushina E, Luetkens H

机构信息

Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute, CH-5232, Villigen PSI, Switzerland.

Laboratory for Multiscale Materials Experiments, Paul Scherrer Institut, 5232, Villigen PSI, Switzerland.

出版信息

Nat Commun. 2023 Nov 28;14(1):7796. doi: 10.1038/s41467-023-43503-9.

Abstract

Charge ordered kagome lattices have been demonstrated to be intriguing platforms for studying the intertwining of topology, correlation, and magnetism. The recently discovered charge ordered kagome material ScVSn does not feature a magnetic groundstate or excitations, thus it is often regarded as a conventional paramagnet. Here, using advanced muon-spin rotation spectroscopy, we uncover an unexpected hidden magnetism of the charge order. We observe an enhancement of the internal field width sensed by the muon ensemble, which takes place within the charge ordered state. More importantly, the muon spin relaxation rate below the charge ordering temperature is substantially enhanced by applying an external magnetic field. Taken together with the hidden magnetism found in AVSb (A = K, Rb, Cs) and FeGe kagome systems, our results suggest ubiqitous time-reversal symmetry-breaking in charge ordered kagome lattices.

摘要

电荷有序的 Kagome 晶格已被证明是研究拓扑、关联和磁性相互交织的有趣平台。最近发现的电荷有序 Kagome 材料 ScVSn 不具有磁性基态或激发态,因此它通常被视为传统顺磁体。在这里,我们使用先进的μ子自旋旋转光谱技术,揭示了电荷有序态中意想不到的隐藏磁性。我们观察到μ子系综所感知的内场宽度增强,这发生在电荷有序态内。更重要的是,通过施加外部磁场,电荷有序温度以下的μ子自旋弛豫率显著增强。结合在 AVSb(A = K、Rb、Cs)和 FeGe Kagome 系统中发现的隐藏磁性,我们的结果表明电荷有序 Kagome 晶格中普遍存在时间反演对称性破缺。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/318e/10684576/24b59637ecbb/41467_2023_43503_Fig1_HTML.jpg

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