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高达11吉帕高压下ScVSn中电荷密度波的失稳与超导性的缺失

Destabilization of the Charge Density Wave and the Absence of Superconductivity in ScVSn under High Pressures up to 11 GPa.

作者信息

Zhang Xiaoxiao, Hou Jun, Xia Wei, Xu Zhian, Yang Pengtao, Wang Anqi, Liu Ziyi, Shen Jie, Zhang Hua, Dong Xiaoli, Uwatoko Yoshiya, Sun Jianping, Wang Bosen, Guo Yanfeng, Cheng Jinguang

机构信息

Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.

School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100190, China.

出版信息

Materials (Basel). 2022 Oct 21;15(20):7372. doi: 10.3390/ma15207372.

Abstract

VSn ( = Sc, Y, or rare earth) is a new family of kagome metals that have a similar vanadium structural motif as VSb ( = K, Rb, Cs) compounds. Unlike VSb, ScVSn is the only compound among the series of VSn that displays a charge density wave (CDW) order at ambient pressure, yet it shows no superconductivity (SC) at low temperatures. Here, we perform a high-pressure transport study on the ScVSn single crystal to track the evolutions of the CDW transition and to explore possible SC. In contrast to VSb compounds, the CDW order of ScVSn can be suppressed completely by a pressure of about 2.4 GPa, but no SC is detected down to 40 mK at 2.35 GPa and 1.5 K up to 11 GPa. Moreover, we observed that the resistivity anomaly around the CDW transition undergoes an obvious change at ~2.04 GPa before it vanishes completely. The present work highlights a distinct relationship between CDW and SC in ScVSn in comparison with the well-studied VSb.

摘要

VSn(= Sc、Y或稀土元素)是一类新型的 Kagome 金属,其具有与VSb(= K、Rb、Cs)化合物相似的钒结构 motif。与VSb不同,ScVSn是VSn系列中唯一在常压下显示电荷密度波(CDW)序的化合物,但在低温下不显示超导性(SC)。在此,我们对ScVSn单晶进行了高压输运研究,以追踪CDW转变的演变并探索可能的超导性。与VSb化合物相比,ScVSn的CDW序在约2.4 GPa的压力下可被完全抑制,但在2.35 GPa和1.5 K至11 GPa的压力下,直至40 mK均未检测到超导性。此外,我们观察到CDW转变附近的电阻率异常在约2.04 GPa时发生明显变化,然后才完全消失。与已充分研究的VSb相比,本工作突出了ScVSn中CDW与超导性之间的独特关系。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/11ba/9611248/687ede65f256/materials-15-07372-g001a.jpg

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