Liu Chen, Zhang Senfu, Hao Hongyuan, Algaidi Hanin, Ma Yinchang, Zhang Xi-Xiang
Physical Science and Engineering Division (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia.
Key Laboratory for Magnetism and Magnetic Materials of the Ministry of Education, Lanzhou University, Lanzhou, 730000, China.
Adv Mater. 2024 May;36(18):e2311022. doi: 10.1002/adma.202311022. Epub 2024 Feb 4.
2D van der Waals (vdW) ferromagnetic crystals are a promising platform for innovative spintronic devices based on magnetic skyrmions, thanks to their high flexibility and atomic thickness stability. However, room-temperature skyrmion-hosting vdW materials are scarce, which poses a challenge for practical applications. In this study, a chemical vapor transport (CVT) approach is employed to synthesize FeGaTe crystals and room-temperature Néel skyrmions are observed in FeGaTe nanoflakes above 58 nm in thickness through in situ Lorentz transmission electron microscopy (L-TEM). Upon an optimized field cooling procedure, zero-field hexagonal skyrmion lattices are successfully generated in nanoflakes with an extended thickness range (30-180 nm). Significantly, these skyrmion lattices remain stable up to 355 K, setting a new record for the highest temperature at which skyrmions can be hosted. The research establishes FeGaTe as an emerging above-room-temperature skyrmion-hosting vdW material, holding great promise for future spintronics.
二维范德华(vdW)铁磁晶体因其高柔韧性和原子厚度稳定性,是基于磁斯格明子的创新自旋电子器件的一个有前景的平台。然而,室温下承载斯格明子的vdW材料稀缺,这对实际应用构成了挑战。在本研究中,采用化学气相传输(CVT)方法合成了FeGaTe晶体,并通过原位洛伦兹透射电子显微镜(L-TEM)在厚度超过58 nm的FeGaTe纳米片中观察到室温奈尔斯格明子。经过优化的场冷程序后,在厚度范围为30-180 nm的纳米片中成功生成了零场六角斯格明子晶格。值得注意的是,这些斯格明子晶格在高达355 K的温度下仍保持稳定,创造了斯格明子能够存在的最高温度的新纪录。该研究将FeGaTe确立为一种新兴的高于室温承载斯格明子的vdW材料,对未来的自旋电子学具有巨大潜力。