Pucher Thomas, Bastante Pablo, Parenti Federico, Xie Yong, Dimaggio Elisabetta, Fiori Gianluca, Castellanos-Gomez Andres
Materials Science Factory. Instituto de Ciencia de Materiales de Madrid (ICMM-CSIC), Madrid, 28049 Spain.
Departamento de Física de la Materia Condensada, Universidad Autónoma de Madrid, 28049 Madrid, Spain.
NPJ 2D Mater Appl. 2023;7(1):73. doi: 10.1038/s41699-023-00436-7. Epub 2023 Nov 3.
This work demonstrates the fabrication and characterization of single-layer MoS field-effect transistors using biodegradable albumen (chicken eggwhite) as gate dielectric. By introducing albumen as an insulator for MoS transistors high carrier mobilities (up to ~90 cm V s) are observed, which is remarkably superior to that obtained with commonly used SiO dielectric which we attribute to ionic gating due to the formation of an electric double layer in the albumen MoS interface. In addition, the investigated devices are characterized upon illumination, observing responsivities of 4.5 AW (operated in photogating regime) and rise times as low as 52 ms (operated in photoconductivity regime). The presented study reveals the combination of albumen with van der Waals materials for prospective biodegradable and biocompatible optoelectronic device applications. Furthermore, the demonstrated universal fabrication process can be easily adopted to fabricate albumen-based devices with any other van der Waals material.
这项工作展示了使用可生物降解的蛋白(鸡蛋清)作为栅极电介质来制造和表征单层MoS场效应晶体管。通过引入蛋白作为MoS晶体管的绝缘体,观察到了高载流子迁移率(高达~90 cm² V⁻¹ s⁻¹),这明显优于使用常用SiO₂电介质所获得的迁移率,我们将其归因于在蛋白-MoS界面形成双电层导致的离子门控。此外,所研究的器件在光照下进行了表征,观察到在光门控模式下的响应度为4.5 A W⁻¹,在光电导模式下的上升时间低至52 ms。本研究揭示了蛋白与范德华材料相结合用于未来可生物降解和生物相容的光电器件应用。此外,所展示的通用制造工艺可以很容易地用于制造基于蛋白与任何其他范德华材料的器件。