Department of Chemistry, Materials, and Chemical Engineering "Giulio Natta", Politecnico di Milano, Piazza L. Da Vinci 32, 20131 Milano, Italy.
INSTM, National Consortium of Materials Science and Technology, Local Unit Politecnico di Milano, 50121 Milano, Italy.
Int J Mol Sci. 2024 May 28;25(11):5888. doi: 10.3390/ijms25115888.
Cyclodextrins (CDs) are cyclic oligosaccharides able to form noncovalent water-soluble complexes useful in many different applications for the solubilization, delivery, and greater bioavailability of hydrophobic drugs. The complexation of 5-fluorouracil (5-FU) with natural or synthetic cyclodextrins permits the solubilization of this poorly soluble anticancer drug. In this theoretical work, the complexes between β-CD and 5-FU are investigated using molecular mechanics (MM) and molecular dynamics (MD) simulations in water. The inclusion complexes are formed thanks to the favorable intermolecular interactions between β-CD and 5-FU. Both 1:1 and 1:2 β-CD/5-FU stoichiometries are investigated, providing insight into their interaction geometries and stability over time in water. In the 1:2 β-CD/5-FU complexes, the intermolecular interactions affect the drug's mobility, suggesting a two-step release mechanism: a fast release for the more exposed and hydrated drug molecule, with greater freedom of movement near the β-CD rims, and a slow one for the less-hydrated and well-encapsulated and confined drug. MD simulations study the intermolecular interactions between drugs and specific carriers at the atomistic level, suggesting a possible release mechanism and highlighting the role of the impact of the drug concentration on the kinetics process in water. A comparison with experimental data in the literature provides further insights.
环糊精(CDs)是环状低聚糖,能够形成非共价水溶性配合物,在增溶、传递和提高疏水性药物的生物利用度方面有许多不同的应用。将 5-氟尿嘧啶(5-FU)与天然或合成环糊精络合,可以增溶这种难溶性抗癌药物。在这项理论工作中,使用分子力学(MM)和分子动力学(MD)模拟在水中研究了β-CD 与 5-FU 之间的配合物。由于β-CD 和 5-FU 之间存在有利的分子间相互作用,形成了包合物。研究了 1:1 和 1:2β-CD/5-FU 两种化学计量比,深入了解了它们在水中的相互作用几何形状和稳定性。在 1:2β-CD/5-FU 配合物中,分子间相互作用影响药物的迁移性,表明存在两步释放机制:对于更暴露和水合的药物分子,快速释放,在β-CD 边缘附近具有更大的自由度,而对于水合程度较低、包裹和限制较好的药物,释放较慢。MD 模拟在原子水平上研究了药物与特定载体之间的分子间相互作用,提出了一种可能的释放机制,并强调了药物浓度对水动力学过程的影响。与文献中的实验数据进行比较,提供了进一步的见解。