Max Planck Institute for the Structure and Dynamics of Matter, Hamburg, Germany.
Max Planck Institute for Solid State Research, Stuttgart, Germany.
Nature. 2024 Aug;632(8023):75-80. doi: 10.1038/s41586-024-07635-2. Epub 2024 Jul 10.
Coherent optical driving in quantum solids is emerging as a research frontier, with many reports of interesting non-equilibrium quantum phases and transient photo-induced functional phenomena such as ferroelectricity, magnetism and superconductivity. In high-temperature cuprate superconductors, coherent driving of certain phonon modes has resulted in a transient state with superconducting-like optical properties, observed far above their transition temperature T and throughout the pseudogap phase. However, questions remain on the microscopic nature of this transient state and how to distinguish it from a non-superconducting state with enhanced carrier mobility. For example, it is not known whether cuprates driven in this fashion exhibit Meissner diamagnetism. Here we examine the time-dependent magnetic field surrounding an optically driven YBaCuO crystal by measuring Faraday rotation in a magneto-optic material placed in the vicinity of the sample. For a constant applied magnetic field and under the same driving conditions that result in superconducting-like optical properties, a transient diamagnetic response was observed. This response is comparable in size with that expected in an equilibrium type II superconductor of similar shape and size with a volume susceptibility χ of order -0.3. This value is incompatible with a photo-induced increase in mobility without superconductivity. Rather, it underscores the notion of a pseudogap phase in which incipient superconducting correlations are enhanced or synchronized by the drive.
相干光学驱动在量子固体中正在成为一个研究前沿,有许多有趣的非平衡量子相和瞬态光诱导功能现象的报道,如铁电性、磁性和超导性。在高温铜酸盐超导体中,某些声子模式的相干驱动导致了具有超导光学性质的瞬态状态,这种状态远高于其转变温度 T 并贯穿赝能隙相。然而,关于这种瞬态状态的微观性质以及如何将其与增强载流子迁移率的非超导状态区分开来,仍存在一些问题。例如,目前尚不清楚以这种方式驱动的铜酸盐是否表现出迈斯纳抗磁性。在这里,我们通过测量置于样品附近的磁光材料中的法拉第旋转,来检查通过光驱动的 YBaCuO 晶体的时变磁场。对于恒定的外加磁场和相同的驱动条件,导致出现类似超导的光学性质,我们观察到瞬态抗磁性响应。该响应的大小与类似形状和尺寸的平衡 II 型超导体在相同体积磁化率 χ 约为-0.3 的情况下的预期值相当。这个值与没有超导性的载流子迁移率的光诱导增加不兼容。相反,它强调了赝能隙相的概念,即初始超导相关性通过驱动得到增强或同步。