Szczepaniak Grzegorz, Kapil Kriti, Adida Samuel, Kim Khidong, Lin Ting-Chih, Yilmaz Gorkem, Murata Hironobu, Matyjaszewski Krzysztof
Department of Chemistry, Carnegie Mellon University, 4400 Fifth Avenue, Pittsburgh, Pennsylvania 15213, United States.
Faculty of Chemistry, University of Warsaw, Pasteura 1, 02-093 Warsaw, Poland.
J Am Chem Soc. 2024 Aug 14;146(32):22247-22256. doi: 10.1021/jacs.4c03675. Epub 2024 Jul 30.
Solid-phase polymer synthesis, historically rooted in peptide synthesis, has evolved into a powerful method for achieving sequence-controlled macromolecules. This study explores solid-phase polymer synthesis by covalently immobilizing growing polymer chains onto a poly(ethylene glycol) (PEG)-based resin, known as ChemMatrix (CM) resin. In contrast to traditional hydrophobic supports, CM resin's amphiphilic properties enable swelling in both polar and nonpolar solvents, simplifying filtration, washing, and drying processes. Combining atom transfer radical polymerization (ATRP) with solid-phase techniques allowed for the grafting of well-defined block copolymers in high yields. This approach is attractive for sequence-controlled polymer synthesis, successfully synthesizing di-, tri-, tetra-, and penta-block copolymers with excellent control over the molecular weight and dispersity. The study also delves into the limitations of achieving high molecular weights due to confinement within resin pores. Moreover, the versatility of the method is demonstrated through its applicability to various monomers in organic and aqueous media. This straightforward approach offers a rapid route to developing tailored block copolymers with unique structures and functionalities.
固相聚合物合成起源于肽合成,如今已发展成为一种用于制备序列可控大分子的强大方法。本研究探索了通过将生长的聚合物链共价固定在基于聚乙二醇(PEG)的树脂(称为ChemMatrix(CM)树脂)上进行固相聚合物合成。与传统的疏水载体不同,CM树脂的两亲性质使其能够在极性和非极性溶剂中溶胀,简化了过滤、洗涤和干燥过程。将原子转移自由基聚合(ATRP)与固相技术相结合,能够以高产率接枝结构明确的嵌段共聚物。这种方法对于序列可控聚合物合成具有吸引力,成功合成了二嵌段、三嵌段、四嵌段和五嵌段共聚物,且对分子量和分散度具有出色的控制。该研究还深入探讨了由于限制在树脂孔内而导致难以实现高分子量的问题。此外,该方法的通用性通过其在有机和水性介质中对各种单体的适用性得到了证明。这种直接的方法为开发具有独特结构和功能的定制嵌段共聚物提供了一条快速途径。