Darkwah-Owusu Victor, Yusof Muhammad Aslam Md, Sokama-Neuyam Yen A, Turkson Joshua N, Fjelde Ingebret
Petroleum Engineering Department, Universiti Teknologi PETRONAS, 32610 Bandar Seri Iskandar, Malaysia; Centre of Reservoir Dynamics (CORED), Institute of Hydrocarbon Recovery, Universiti Teknologi PETRONAS, 32610 Bandar Seri Iskandar, Perak Darul Ridzuan, Malaysia.
Petroleum Engineering Department, Universiti Teknologi PETRONAS, 32610 Bandar Seri Iskandar, Malaysia.
Sci Total Environ. 2024 Nov 10;950:175232. doi: 10.1016/j.scitotenv.2024.175232. Epub 2024 Aug 5.
Geological CO sequestration is a proven method for mitigating climate change by reducing atmospheric CO levels. However, CO injection often induces salt precipitation, leading to decreased formation permeability, which in turn limits CO injectivity and storage capacity. Conventional approaches, such as freshwater and low-salinity water injection, have been employed to mitigate salt precipitation. Despite their widespread use, these methods provide only temporary improvement and can be ineffective in some scenarios, resulting in long-term issues such as salt recrystallization and clay swelling. Given the complexity and significance of this issue, a comprehensive review of salt precipitation mechanisms and remediation techniques is essential. This paper critically examines the processes of salt precipitation during CO injection in saline aquifers and evaluates various remediation techniques aimed at improving CO injectivity. The paper reviews the influence of CO flow dynamics, geochemical reactions, and fluid properties on salt precipitation and pore throat accumulation, assessing the efficacy and limitations of existing mitigation methods. Additionally, the paper explores alternative techniques with potential for long-term CO sequestration, analyzing their advantages and drawbacks. Based on insights from the reviewed sources, the paper recommends exploring alternative treatment measures and the integration of hybrid solutions to enhance CO injectivity. The findings presented serve as a valuable reference for advancing research and practice in this critical area, offering a deeper understanding of the challenges and potential solutions for effective CO sequestration in saline aquifers.
地质二氧化碳封存是一种通过降低大气中二氧化碳水平来缓解气候变化的成熟方法。然而,注入二氧化碳往往会引发盐分沉淀,导致地层渗透率降低,进而限制二氧化碳的注入能力和储存容量。传统方法,如注入淡水和低盐度水,已被用于减轻盐分沉淀。尽管这些方法被广泛使用,但它们只能提供暂时的改善,并且在某些情况下可能无效,从而导致诸如盐再结晶和粘土膨胀等长期问题。鉴于这个问题的复杂性和重要性,对盐分沉淀机制和修复技术进行全面综述至关重要。本文批判性地研究了在盐水层中注入二氧化碳期间的盐分沉淀过程,并评估了旨在提高二氧化碳注入能力的各种修复技术。本文综述了二氧化碳流动动力学、地球化学反应和流体性质对盐分沉淀和孔喉堵塞的影响,评估了现有缓解方法的有效性和局限性。此外,本文探讨了具有长期二氧化碳封存潜力的替代技术,分析了它们的优缺点。基于综述文献的见解,本文建议探索替代处理措施以及整合混合解决方案以提高二氧化碳注入能力。所呈现的研究结果为推进这一关键领域的研究和实践提供了有价值的参考,有助于更深入地理解在盐水层中有效封存二氧化碳所面临的挑战和潜在解决方案。