Meng Qingkai, Dong Jianting, Nie Pan, Xu Liangcai, Wang Jinhua, Jiang Shan, Zuo Huakun, Zhang Jia, Li Xiaokang, Zhu Zengwei, Balents Leon, Behnia Kamran
Wuhan National High Magnetic Field Center and School of Physics, Huazhong University of Science and Technology, Wuhan, 430074, China.
Laboratoire de Physique et d'Etude de Matériaux (CNRS), ESPCI Paris, PSL Research University, 75005, Paris, France.
Nat Commun. 2024 Aug 13;15(1):6921. doi: 10.1038/s41467-024-51268-y.
Whenever the elastic energy of a solid depends on magnetic field, there is a magnetostrictive response. Field-linear magnetostriction implies piezomagnetism and vice versa. Here, we show that MnSn, a non-collinear antiferromanget with Weyl nodes, hosts a large and almost perfectly linear magnetostriction even at room temperature. The longitudinal and transverse magnetostriction, with opposite signs and similar amplitude are restricted to the kagome planes and the out-of-plane response is negligibly small. By studying four different samples with different Mn:Sn ratios, we find a clear correlation between the linear magnetostriction, the spontaneous magnetization and the concentration of Sn vacancies. The recently reported piezomagnetic data fits in our picture. We show that linear magnetostriction and piezomagnetism are both driven by the field-induced in-plane twist of spins. A quantitative account of the experimental data requires the distortion of the spin texture by Sn vacancies. We find that the field-induced domain nucleation within the hysteresis loop corresponds to a phase transition. Within the hysteresis loop, a concomitant mesoscopic modulation of local strain and spin twist angles, leading to twisto-magnetic stripes, arises as a result of the competition between elastic and magnetic energies.
只要固体的弹性能取决于磁场,就会有磁致伸缩响应。场线性磁致伸缩意味着压磁效应,反之亦然。在此,我们表明,具有外尔节点的非共线反铁磁体MnSn即使在室温下也具有大且几乎完美线性的磁致伸缩。纵向和横向磁致伸缩具有相反的符号和相似的幅度,且局限于戈薇平面,而面外响应小到可忽略不计。通过研究四种具有不同Mn:Sn比例的不同样品,我们发现线性磁致伸缩、自发磁化和Sn空位浓度之间存在明显的相关性。最近报道的压磁数据符合我们的描述。我们表明,线性磁致伸缩和压磁效应均由场诱导的面内自旋扭转驱动。对实验数据的定量解释需要考虑Sn空位引起的自旋纹理畸变。我们发现,磁滞回线内场诱导的磁畴成核对应于一个相变。在磁滞回线内,由于弹性能和磁能之间的竞争,出现了局部应变和自旋扭转角的伴随介观调制,从而导致扭转磁条纹。